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Thermoluminescence dosimetry features of DY and Cu doped SrF2 nanoparticles under gamma irradiation

机译:γ和DY掺杂Cu和SrF2纳米粒子的热致发光剂量学特征

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Dy and Cu-doped SrF2 nanoparticles (NPs) were synthesized by using co-precipitation method and their possible application to solid state dosimetry were studied and compared to that of pure SrF2 NPs. X-ray diffraction (XRD), scanning electron microscopy (SEM) and energy dispersive spectrometer (EDS) were used for sample characterization. The highest thermoluminescence (TL) response of SrF2:Dy and SrF2:Cu NPs were found respectively at 0.5 and 0.7 mol% of Dy and Cu impurities. Seven overlapping glow peaks at 384, 406, 421, 449, 569, 495, 508 K and three component glow peaks at 381, 421 and 467 K were identified respectively for SrF2:Dy and SrF2:Cu NPs employing T-m-T-stop and computerized glow curve deconvolution (CGCD) methods. The TL sensitivity of SrF2:Dy is approximately the same as that of LiF:Mg, Ti (TLD-100) cheeps. Linear dose response were observed for the SrF2:Dy and SrF2:Cu NPs up to the absorbed doses of 1 kGy and 10 kGy correspondingly. Regarding other dosimetry characteristics of the produced NPs such as fading, reproducibility and thermal treatment, Dy and Cu doped SrF2 NPs recommend for high dose TL dosimetry applications. (C) 2015 Elsevier Ltd. All rights reserved.
机译:采用共沉淀法合成了Dy和Cu掺杂的SrF2纳米颗粒,并研究了它们在固态剂量学中的应用,并与纯SrF2 NPs进行了比较。 X射线衍射(XRD),扫描电子显微镜(SEM)和能量分散光谱仪(EDS)用于样品表征。发现SrF2:Dy和SrF2:Cu NP的最高热致发光(TL)响应分别在Dy和Cu杂质为0.5和0.7 mol%时出现。对于使用TmT停止和计算机化发光的SrF2:Dy和SrF2:Cu NP,分别在384、406、421、449、569、495、508 K处出现七个重叠辉光峰,在381、421和467 K处确定了三个组分辉光峰。曲线反卷积(CGCD)方法。 SrF2:Dy的TL灵敏度与LiF:Mg,Ti(TLD-100)的低灵敏度大致相同。观察到SrF2:Dy和SrF2:Cu NP的线性剂量反应,分别达到吸收剂量1 kGy和10 kGy。关于所产生的NP的其他剂量学特性,例如褪色,可重复性和热处理,Dy和Cu掺杂的SrF2 NPs建议用于高剂量TL剂量学应用。 (C)2015 Elsevier Ltd.保留所有权利。

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