Radionuclide migration at experimental polygon at Red Forest waste site in Chernobyl zone. Part 2: Hydrogeological characterization and groundwater transport modeling

摘要

This article represents the second of two articles, which review the main results of the international radioecological projects: Chernobyl Pilot Site Project (1999-2003) and Experimental Platform in Chernobyl (2004-2008). These projects studied radionuclide migration from the near-surface radioactive waste trench at the Red Forest waste dump in the Chernobyl zone, which contained nuclear fuel particles. This article presents results from the comprehensive hydrogeological site characterization program including the following issues: geological structure of the study site, hydraulic properties of the deposits, tracer tests in the aquifer, results of groundwater monitoring and unsaturated zone regime studies, as well as data on the ~(90)Sr distribution in the unsaturated zone and aquifer, and analyses of ~(90))Sr sorption behavior. The derived parameters were used to develop and calibrate 1D (flow tube) and 2D (cross-section) models describing the migration of ~(90)Sr from the studied waste trench to the unsaturated zone and aquifer over a 16-a period (1986-2002). The models involved the following sub-models: (1) the geostatistical (structural) model for radioactivity distribution in the trench (using GSLIB); and (2) the radionuclide source term model (STERM1D) describing dissolution of fuel particles and a 1D of radionuclide redistribution in the trench body and unsaturated zone. The MODFLOW - MT3D codes were used to model the 2D ~(90)Sr transport in the aquifer cross-section. Calibration of the 1D model with respect to K _ds and dispersivities allowed quite accurate reproduction of ~(90)Sr migration behavior for the early period (1995-1998). The less perfect fit between the 1D and 2D modeling results and monitoring data for the later period (1999-2002) suggests the need to improve the conceptual radionuclide migration model (i.e. to account for transient hydraulic and geochemical regimes of the waste site).