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Electrosynthesis of a Defective Indium Selenide with 3D?Structure on a Substrate for Tunable CO2 Electroreduction to Syngas

机译：用于3D型硒化型有缺陷铟硒化型的电动合成衬底上的结构，用于合成气的基板上

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Abstract > Syngas (CO/H <sub>2</sub> ) is a feedstock for the production of a variety of valuable chemicals and liquid fuels, and CO <sub>2</sub> electrochemical reduction to syngas is very promising. However, the production of syngas with high efficiency is difficult. Herein, we show that defective indium selenide synthesized by an electrosynthesis method on carbon paper (γ‐In <sub>2</sub> Se <sub>3</sub> /CP) is an extremely efficient electrocatalyst for this reaction. CO and H <sub>2</sub> were the only products and the CO/H <sub>2</sub> ratio could be tuned in a wide range by changing the applied potential or the composition of the electrolyte. In particular, using nanoflower‐like γ‐In <sub>2</sub> Se <sub>3</sub> /CP (F‐γ‐In <sub>2</sub> Se <sub>3</sub> /CP) as the electrode, the current density could be as high as 90.1?mA?cm ?2 at a CO/H <sub>2</sub> ratio of 1:1. In addition, the Faradaic efficiency of CO could reach 96.5?% with a current density of 55.3?mA?cm ?2 at a very low overpotential of 220?mV. The outstanding electrocatalytic performance of F‐γ‐In <sub>2</sub> Se <sub>3</sub> /CP can be attributed to its defect‐rich 3D?structure and good contact with the CP substrate. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 合成气（CO / H. <sub> 2 </ sub> ）生产各种有价值的化学品和液体燃料的原料，以及CO <sub> 2 </ sub> 电化学减少到合成气是非常有前途的。但是，难以生产高效率的合成气。在此，我们表明，通过电气合成方法在碳纸上合成了缺陷硒化型（γ- <sub> 2 </ sub> se <sub> 3 </ sub> / cp）是这种反应的极其有效的电催化剂。 CO和H. <sub> 2 </ sub> 是唯一的产品和co / h <sub> 2 </ sub> 通过改变施加的电位或电解质的组成，可以在宽范围内调谐比率。特别是，使用纳米闪光样γ-in <sub> 2 </ sub> se <sub> 3 </ sub> / cp（f-γ-in <sub> 2 </ sub> se <sub> 3 </ sub> / cp）作为电极，电流密度可以高达90.1？ma？cm ？2 </ sup> 在一个co / h <sub> 2 </ sub> 比例为1：1。此外，CO的法拉迪效率可以达到96.5？％，电流密度为55.3？ma？cm ？2 </ sup> 在220的非常低的过电位下。 F-γ-in的出色电催化性能 <sub> 2 </ sub> se <sub> 3 </ sub> / CP可归因于其缺陷的3D？结构和与CP基板良好接触。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-19011/'>《Angewandte Chemie》</a> <b style="margin: 0 2px;">|</b><span>2020年第6期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Dexin&option=202" target="_blank" rel="nofollow">Yang Dexin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhu Qinggong&option=202" target="_blank" rel="nofollow">Zhu Qinggong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sun Xiaofu&option=202" target="_blank" rel="nofollow">Sun Xiaofu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Chunjun&option=202" target="_blank" rel="nofollow">Chen Chunjun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Guo Weiwei&option=202" target="_blank" rel="nofollow">Guo Weiwei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Guanying&option=202" target="_blank" rel="nofollow">Yang Guanying;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Han Buxing&option=202" target="_blank" rel="nofollow">Han Buxing;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Beijing National Laboratory for Molecular SciencesChinese Academy of SciencesBeijing 100190 China;</p> <p>Beijing National Laboratory for Molecular SciencesChinese Academy of SciencesBeijing 100190 China;</p> <p>Beijing National Laboratory for Molecular SciencesChinese Academy of SciencesBeijing 100190 China;</p> <p>Beijing National Laboratory for Molecular SciencesChinese Academy of SciencesBeijing 100190 China;</p> <p>Beijing National Laboratory for Molecular SciencesChinese Academy of SciencesBeijing 100190 China;</p> <p>Beijing National Laboratory for Molecular SciencesChinese Academy of SciencesBeijing 100190 China;</p> <p>Beijing National Laboratory for Molecular SciencesChinese Academy of SciencesBeijing 100190 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1188.html" title="应用化学">应用化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=CO2 reduction&option=203" rel="nofollow">CO2 reduction;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrocatalysis&option=203" rel="nofollow">electrocatalysis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=indium selenide&option=203" rel="nofollow">indium selenide;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=ionic liquid&option=203" rel="nofollow">ionic liquid;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=syngas production&option=203" rel="nofollow">syngas production;</a> </p> <div class="translation"> 机译：二氧化碳减少;电催化;硒化铟;离子液体;合成气生产; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704028162261.html">Electrosynthesis of a Defective Indium Selenide with 3D?Structure on a Substrate for Tunable CO2 Electroreduction to Syngas</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Dexin&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Yang Dexin,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhu Qinggong&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Zhu Qinggong,</a> <a 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