Optimizing pink‐beam fast X‐ray microtomography for multiphase flow in 3D porous media

摘要

Summary A fast pink‐beam X‐ray microtomography methodology was developed at the GSECARS 13‐BMD beamline at the Advanced Photon Source to study multiphase flow in porous media. The white beam X‐ray distribution of the Advanced Photon Source is modified using a 1‐mm copper filter and the beam is reflected off a platinum mirror angled at 1.5 mrad, resulting in a pink beam with X‐ray intensities predominately in the range of 40–60 keV. Bubble formation in the wetting phase and wettability alteration of the solid phase from x‐ray exposure can be a problem with high flux and high energy beams, but the suggested pink‐beam configuration mitigates these effects. With a 14‐second acquisition time for capturing a complete dataset, the evolving fluid‐fronts of nonequilibrium three‐dimensional multiphase flow can be studied in real‐time and the images contain adequate image contrast and quality to measure important multiphase quantities such as contact angles and interfacial areas. Lay Description Understanding how fluids are transported through porous materials is pertinent to many important societal processes in the environment (e.g. groundwater flow for drinking water) and industry (e.g. drying of industrial materials such as pulp and paper). To develop accurate models and theories of this fluid transportation, experiments need to track fluids in 3‐dimensions quickly. This is difficult to do as most materials are opaque and therefore cameras cannot capture fluid movement directly. But, with the help of x‐rays, scientists can track fluids in 3D using an imaging technique called x‐ray microtomography (μCT). Standard μCT takes about 15 minutes for one image which can produce blurry images if fluids are flowing quickly through the material. We present a technique, fast μCT, which uses a larger spectrum of x‐rays than the standard technique and acquires a 3D image in 14 seconds. With the large amount of x‐rays utilized in this technique, bubbles can start to form in the fluids from x‐ray exposure. We optimized the utilized x‐ray spectrum to limit bubble formation while still achieving a rapid 3D image acquisition that has adequate image quality and contrast. With this technique, scientists can study fluid transport in 3D porous materials in near real‐time for the improvement of models used to ensure public and environmental health.