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Recent advances and future prospect in catalysts for oxidative coupling of methane to ethylene: A review

机译:甲烷氧化偶联催化剂的最新进展和未来前景乙烯乙烯:综述

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Despite its inherent constraints which hindered significant improvement in the process catalytically, the oxidative coupling of methane (OCM) remains an indispensable prospective approach for converting methane directly into vital chemicals such as ethylene. Recently, there is an upsurge in research effort towards better understanding of the oxidative coupling of methane process in terms of its mechanism, catalyst design and synthesis. This review discusses recent advances in crucial aspects related to the catalyst such as active sites, oxygen vacancy, acid-base property, surface oxide reducibility, oxide support interaction, and prospects of nanowires with the aim to improve the performance of the OCM process. (C) 2017 The Korean Society of Industrial and Engineering Chemistry. Published by Elsevier B.V. All rights reserved.
机译:尽管其固有的约束致力于催化过程中的重大改善,但甲烷(OCM)的氧化偶联仍然是将甲烷直接转化为乙烯等重要化学品的不可或缺的前瞻性方法。 最近,在其机理,催化剂设计和合成方面更好地了解甲烷过程的氧化偶联的研究努力有一种高潮。 本综述讨论了与催化剂如活性位点,氧空位,酸碱性,表面氧化物还原性,氧化物载体相互作用,氧化物载体相互作用等关键方面进行了最近的进展,并旨在改善OCM工艺的性能。 (c)2017年韩国工程和工程化学学会。 elsevier b.v出版。保留所有权利。

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