Concentrations and cycling of DMS, DMSP, and DMSO in coastal and offshore waters of the Subarctic Pacific during summer, 2010‐2011

Asher Elizabeth; Dacey John W.; Ianson Debby; Pe?a Angelica; Tortell Philippe D.

摘要

Abstract > Concentrations of dimethylsulfide (DMS), measured in the Subarctic Pacific during summer 2010 and 2011, ranged from ～1 to 40 nM, while dissolved dimethylsulfoxide (DMSO) concentrations (range 13‐23 nM) exceeded those of dissolved dimethyl sulfoniopropionate (DMSP) (range 1.3–8.8 nM). Particulate DMSP dominated the reduced sulfur pool, reaching maximum concentrations of 100 nM. Coastal and off shore waters exhibited similar overall DMS concentration ranges, but sea‐air DMS fluxes were lower in the oceanic waters due to lower wind speeds. Surface DMS concentrations showed statistically significant correlations with various hydrographic variables including the upwelling intensity (r 2 ?=?0.52, p ??0.001) and the Chlorophyll a /mixed layer depth ratio (r 2 ?=?0.52, p ??0.001), but these relationships provided little predictive power at small scales. Stable isotope tracer experiments indicated that the DMSP cleavage pathway always exceeded the DMSO reduction pathway as a DMS source, leading to at least 85% more DMS production in each experiment. Gross DMS production rates were positively correlated with the upwelling intensity, while net rates of DMS production were significantly correlated to surface water DMS concentrations. This latter result suggests that our measurements captured dominant processes driving surface DMS accumulation across a coastal‐oceanic gradient. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><abstract xmlns =“http://www.wiley.com/namespaces/wiley”type =“main”> <标题类型=“main”>抽象</ title> > 在2010年夏季和2011年夏季太平洋（DMS）中测量的二甲基硫醚（DMS）的浓度范围为约1至40nm，而溶解的二甲基磺酰氧化物（DMSO）浓度（范围为13-23nm）超过溶解的二甲基磺基丙酸酯（DMSP）（范围1.3-8.8 nm）。颗粒状DMSP占据了还原的硫池，达到了100nm的最大浓度。沿海和岸边的水域展出了类似的总体DMS浓度范围，但由于风速较低，海洋水域较低。表面DMS浓度显示出与各种水文变量的统计学相关性，包括升值强度（R 2 </ sup> ？=？0.52， p </ i> ？＆？0.001）和叶绿素 a </ i> /混合层深度比（r 2 </ sup> ？=？0.52， p </ i> ？＆？0.001），但这些关系在小尺度上提供了很少的预测力。稳定的同位素示踪剂实验表明，DMSP裂解途径总是超过DMSO还原途径作为DMS源，在每个实验中产生至少85％的DMS产生。总DMS生产率与上升强度正相关，而DMS产量的净率与表面水DMS浓度显着相关。后一种结果表明，我们的测量捕获了沿海海洋梯度的主导过程驱动表面DMS积累。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" > 著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-34643/'>《Journal of Geophysical Research, C. Oceans: JGR 》</a> <b style="margin: 0 2px;">|</b><span>2017年第4期</span><b style="margin: 0 2px;">|</b> <span>共18页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Asher Elizabeth&option=202" target="_blank" rel="nofollow">Asher Elizabeth;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dacey John W.&option=202" target="_blank" rel="nofollow">Dacey John W.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ianson Debby&option=202" target="_blank" rel="nofollow">Ianson Debby;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Pe?a Angelica&option=202" target="_blank" rel="nofollow">Pe?a Angelica;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tortell Philippe D.&option=202" target="_blank" rel="nofollow">Tortell Philippe D.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Earth Ocean and Atmospheric SciencesUniversity of British ColumbiaVancouver British Columbia Canada;</p> <p>Biology DepartmentWoods Hole Oceanographic InstitutionWoods Hole Massachusetts USA;</p> <p>Department of Earth Ocean and Atmospheric SciencesUniversity of British ColumbiaVancouver British Columbia Canada;</p> <p>Institute of Ocean Sciences Fisheries and Oceans CanadaSidney British Columbia Canada;</p> <p>Department of Earth Ocean and Atmospheric SciencesUniversity of British ColumbiaVancouver British Columbia Canada;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li> <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span> <a href="https://www.zhangqiaokeyan.com/clc/163.html" title="地球物理学">地球物理学 ;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=dimethylsulfide&option=203" rel="nofollow">dimethylsulfide;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=DMSP&option=203" rel="nofollow">DMSP;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=DMSO&option=203" rel="nofollow">DMSO;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=DMS turnover&option=203" rel="nofollow">DMS turnover;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=rate measurements&option=203" rel="nofollow">rate measurements;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=isotopic tracers&option=203" rel="nofollow">isotopic tracers;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=sea‐air flux&option=203" rel="nofollow">sea‐air flux;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=upwelling&option=203" rel="nofollow">upwelling;</a> </p> <div class="translation"> 机译：二甲基硫化物;DMSP;DMSO;DMS营业额;速率测量;同位素示踪剂;海空气助焊剂;升值; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704025579025.html">Concentrations and cycling of DMS, DMSP, and DMSO in coastal and offshore waters of the Subarctic Pacific during summer, 2010‐2011</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Asher Elizabeth&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Asher Elizabeth,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dacey John W.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Dacey John W.,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ianson Debby&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Ianson Debby,</a> <a href="/journal-foreign-34643/" target="_blank" rel="nofollow" class="tuijian_authcolor">Journal of Geophysical Research, C. 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href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=夏辉&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,夏辉</a> <span> <a href="/journal-cn-7204/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 水产学报 </a> </span> <span> . 2013</span><span> ,第009期</span> </span> </div> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/academic-journal-cn_acta-oceanologica-sinica_thesis/0201253882208.html">2010-2011年长江河口及邻近水域春夏季仔稚鱼群落结构及其多样性的研究</a> <b>[J]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=蒋玫&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 蒋玫</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=李磊&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,李磊</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=沈新强&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,沈新强</a> <span> <a href="/journal-cn-4977/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 海洋学报（中文版） </a> </span> <span> . 2014</span><span> ,第006期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-14539_thesis/020221172090.html">夏季亚洲——太平洋涛动与我国近海热带气旋活动的关系</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=邹燕&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 邹燕</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=赵平&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,赵平</a> <span> <a href="/conference-cn-14539/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 2009年福建省气象学会学术年会——省科协第九届学术年会卫星会议 </a> <span> <span> . 2009</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020311523921.html">2011年春、夏季广西近海浮游动物群落特征研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=潘非斐&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 潘非斐</a> <span> . 2012</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120211941771.html">一种沿海水域冲锋舟用配件箱</a> <b>[P]</b> . <span> 中国专利： CN211918931U </span> <span> . 2020-11-13</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/061201783901.html">一种异育银鲫在沿海盐碱水域池塘高产养殖方法</a> <b>[P]</b> . <span> 中国专利： CN103283641B </span> <span> . 2015.10.21</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130441377934.html">Topical composition containing dimethyl sulfoxide (DMSO) and dexapanthenol, useful for treating e.g. injuries and rheumatic disease, can contain high concentration of DMSO without causing skin irritation</a> <b>[P]</b> . <span> 外国专利：  DE20319986U1 </span> <span> . 2004-05-19</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：包含二甲基亚砜（DMSO）和右旋黄腐酚的局部组合物，可用于治疗例如受伤和风湿病，可能含有高浓度的DMSO而不会引起皮肤刺激 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130441377935.html">Topical composition containing dimethyl sulfoxide (DMSO) and dexapanthenol, useful for treating e.g. injuries and rheumatic disease, can contain high concentration of DMSO without causing skin irritation</a> <b>[P]</b> . <span> 外国专利：  DE20319986U1 </span> <span> . 2004-04-15</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：包含二甲基亚砜（DMSO）和右旋黄腐酚的局部组合物，可用于治疗例如受伤和风湿病，可能含有高浓度的DMSO而不会引起皮肤刺激 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130449179902.html">TREATMENT APPARATUS OF DMSO-CONTAINING WATER AND TREATMENT EQUIPMENT OF WASTE WATER OF SEMICONDUCTOR FACTORY</a> <b>[P]</b> . <span> 外国专利：  JP2000350993A </span> <span> . 2000-12-19</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：含DMSO的水处理装置及半导体厂废水处理设备 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704025579025','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div 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