Ozonation inactivation of <fc xmlns='http://www.wiley.com/namespaces/wiley'> <fi>Escherichia coli</fi> </fc> <fi xmlns='http://www.wiley.com/namespaces/wiley'>Escherichia coli</fi>Escherichia coli in aqueous solution over MgO nanocrystals: modelling and mechanism

Chen Jun; Xu Shuang; Yang Hai; Au Chaktong; Tian Shuanghong; Xiong Ya

摘要

Abstract <section xml:id="jctb5535-sec-0001" numbered="no"> <title type="main" xml:lang="de">BACKGROUND >This study aims to reveal the potential of using heterogeneous catalytic ozonation processes (HCOP) in water disinfection and provide a direction to tailor the catalytic activity by crystal facet engineering. Four kinds of MgO nanocrystals individually with exposure of (111), (200), (110) and (100) facets were prepared and used. </section> <section xml:id="jctb5535-sec-0002" numbered="no"> <title type="main">RESULTS > It is found that MgO functions as a bactericide as well as a catalyst for ozonation. The catalytic activity of MgO nanocrystals decreases in the order MgO(111)??MgO(200)??MgO(110)??MgO(100). The apparent first‐order inactivation rate (k <sub>ap</sub> ) fitted by the Hom model of MgO(111)/O <sub>3</sub> is 2.56?min ‐1 , which is 32.0 and 3.5 times that of single ozonation and classic MgO(100)/O <sub>3</sub> . It is confirmed by scavenger studies that ?OH mainly works in MgO(111)/O <sub>3</sub> while more direct ozonation occurs in other cases. Some O <sub>2</sub> ?? are also detected in the presence of MgO. With the attack of these reactive oxidation species, cell membranes were damaged and intracellular components were released, leading to the death of <fc> <fi>Escherichia coli</fi> </fc> . </section> <section xml:id="jctb5535-sec-0003" numbered="no"> <title type="main">CONCLUSION >These results indicate that HCOP is a promising technology for water disinfection, and c </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <title type =“main”>抽象</ title> <section XML：ID =“JCTB5535-SEC-0001”编号=“否”> <标题类型=“main”XML：lang =“de”>背景</ title> >本研究旨在揭示使用异质催化臭氧化过程的潜力（HCOP）在水消毒中，并提供了通过水晶面工程定制催化活性的方向。使用（111），（200），（110）和（100）个刻面的暴露单独进行四种MgO纳米晶体。</ p> </ section> <章节XML：ID =“JCTB5535-SEC-0002 “编号=”否“> <标题类型=”main“>结果</标题> >发现MgO用作杀菌剂以及臭氧化催化剂。 MgO纳米晶体的催化活性在MgO（111）中减少（111）？MgO（200）？MgO（110）？＆？MgO（100）。 MgO（111）/ O <Sub> 3 </ sub> HOM模型配位的表观一阶失活率（K <sub> ap </ sub>）为2.56Ω·min -1 </ sup >，单次臭氧和经典MgO（100）/ O <亚> 3 </ sub>的32.0和3.5倍。通过清除剂研究证实了吗？OH主要在MgO（111）/ O <sub> 3 </ sub>，而在其他情况下发生更多的直接臭氧。在MgO的存在下，还检测到一些O <sub> 2 </ sub> Δθ。随着这些反应性氧化物种的攻击，细胞膜被损坏，释放细胞内部件，导致<FC> <FI>大肠杆菌的死亡。 </ p> </ section> <section XML：ID =“JCTB5535-SEC-0003”编号=“否”> <标题类型=“main”>结论</ title> >这些结果表明HCOP是一个有希望的水消毒技术和C. </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-33908/'>《Journal of Chemical Technology & Biotechnology》</a> <b style="margin: 0 2px;">|</b><span>2018年第6期</span><b style="margin: 0 2px;">|</b><span>共7页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Jun&option=202" target="_blank" rel="nofollow">Chen Jun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Shuang&option=202" target="_blank" rel="nofollow">Xu Shuang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Hai&option=202" target="_blank" rel="nofollow">Yang Hai;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Au Chaktong&option=202" target="_blank" rel="nofollow">Au Chaktong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tian Shuanghong&option=202" target="_blank" rel="nofollow">Tian Shuanghong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xiong Ya&option=202" target="_blank" rel="nofollow">Xiong Ya;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>School of Environmental Science and EngineeringSun Yat‐sen UniversityGuangzhou PR China;</p> <p>School of Environmental Science and EngineeringSun Yat‐sen UniversityGuangzhou PR China;</p> <p>College of Chemistry and Chemical EngineeringHunan Institute of EngineeringXiangtan PR China;</p> <p>College of Chemistry and Chemical EngineeringHunan Institute of EngineeringXiangtan PR China;</p> <p>School of Environmental Science and EngineeringSun Yat‐sen UniversityGuangzhou PR China;</p> <p>School of Environmental Science and EngineeringSun Yat‐sen UniversityGuangzhou PR China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/180.html" title="生物工程学（生物技术）">生物工程学（生物技术）;</a><a href="https://www.zhangqiaokeyan.com/clc/20827.html" title="生物化学过程">生物化学过程;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=MgO&option=203" rel="nofollow">MgO;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=crystal facet&option=203" rel="nofollow">crystal facet;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=catalytic ozonation&option=203" rel="nofollow">catalytic ozonation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Escherichia coli&option=203" rel="nofollow">Escherichia coli;</a> </p> <div class="translation"> 机译：MgO;水晶面;催化臭氧化;大肠杆菌; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704025422885.html">Ozonation inactivation of <fc xmlns="http://www.wiley.com/namespaces/wiley"> <fi>Escherichia coli</fi> </fc> <fi xmlns="http://www.wiley.com/namespaces/wiley">Escherichia coli</fi>Escherichia coli in aqueous solution over MgO nanocrystals: modelling and mechanism</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chen Jun&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Chen Jun,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu 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Ozonation inactivation of Escherichia coli Escherichia coliEscherichia coli in aqueous solution over MgO nanocrystals: modelling and mechanism

摘要