Hot Spot Chemistry in Several Polymer‐Bound Explosives under Nanosecond Shock Conditions

Bassett Will P.; Johnson Belinda P.; Dlott Dana D.

摘要

Abstract > Initial hot spot temperatures and temperature evolutions for 4 polymer‐bound explosives under shock compression by laser‐driven flyer plates at speeds from 1.5–4.5?km?s ?1 are presented. A new averaging routine allows for improved signal to noise in shock compressed impactor experiments and yields temperature dynamics which are more accurate than has been previously available. The PBX formulations studied here consist of either pentaerythritol tetranitrate (PETN), 1,3,5‐trinitro‐1,3,5‐triazinane (RDX), 2,4,6‐trinitrotoluene (TNT), or 1,3,5‐triamino‐2,4,6‐trinitrobenzene (TATB) in a 80/20?wt.% mixture with a silicone elastomer binder. The temperature dynamics demonstrate a unique shock strength dependence for each base explosive. The initial hot spot temperature and its evolution in time are shown to be indicative of chemistry occurring within the reaction zone of the four explosives. The number density of hot spots is qualitatively inferred from the spatially‐averaged emissivity and appears to increase exponentially with shock strength. An increased emissivity for formulations consisting of TNT and TATB is consistent with carbon‐rich explosives and in increased hot spot volume. Qualitative conclusions about sensitivity were drawn from the initial hot spot temperature and rate at which the number of hot spots appear to grow. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 初始热点温度和4种聚合物爆炸物的温度演进，通过激光驱动的飞行器在1.5-4.5Ωm的速度下通过激光驱动的飞行器板进行冲击压缩？1 </ sup> 呈现。新的平均例程允许改进的信号在冲击压缩撞击器实验中提高信号，并产生比以前可用的更准确的温度动态。研究的PBX制剂包括季戊四醇四硝酸酯（PETN），1,3,5-三腈-1,3,5-三嗪（RDX），2,4,6-三硝基甲苯（TNT），或1,3,5 - 在80/20的氧化铝-2,4,6-三硝基苯（TATB）中的80/20？重量％。用硅氧烷弹性体粘合剂的％混合物。温度动力学表现出对每个碱爆炸的独特冲击力依赖性。最初的热点温度及其在时间的演变中显示出在四种炸药的反应区内发生化学。热点的数量密度从空间平均发射率定性推断，似乎随着休克强度指数增加。由TNT和TATB组成的配方的增加的发射率与富含碳爆炸物和增加的热点体积一致。关于灵敏度的定性结论是从初始热点温度和热点数量似乎生长的速率中得出的。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-29946/'>《Propellants, Explosives, Pyrotechnics》</a> <b style="margin: 0 2px;">|</b><span>2020年第2期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Bassett Will P.&option=202" target="_blank" rel="nofollow">Bassett Will P.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Johnson Belinda P.&option=202" target="_blank" rel="nofollow">Johnson Belinda P.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Dlott Dana D.&option=202" target="_blank" rel="nofollow">Dlott Dana D.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Energetic Materials CenterLawrence Livermore National Laboratory7000 East Ave Livermore CA 94550 USA;</p> <p>School of Chemical Sciences and Fredrick Seitz Materials Research LaboratoryUniversity of Illinois at Urbana-ChampaignUrbana Il 61801 USA;</p> <p>School of Chemical Sciences and Fredrick Seitz Materials Research LaboratoryUniversity of Illinois at Urbana-ChampaignUrbana Il 61801 USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1837.html" title="爆炸物工业、火柴工业">爆炸物工业、火柴工业;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=PBX&option=203" rel="nofollow">PBX;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Pyrometry&option=203" rel="nofollow">Pyrometry;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Emission Spectra&option=203" rel="nofollow">Emission Spectra;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=PETN&option=203" rel="nofollow">PETN;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=RDX&option=203" rel="nofollow">RDX;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=TNT&option=203" rel="nofollow">TNT;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=TATB&option=203" rel="nofollow">TATB;</a> </p> <div class="translation"> 机译：PBX;热尺寸;发射光谱;佩特;RDX;TNT;TATB; 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href="/journal-cn-8453/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 原子能科学技术 </a> </span> <span> . 2019</span><span>,第008期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-12078_thesis/02022546504.html">几种分步压装用炸药在撞击条件下的热响应研究</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=董军&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 董军</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=赵省向&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,赵省向</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=徐洪涛&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,徐洪涛</a> <span> <a href="/conference-cn-12078/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 2010年火炸药技术学术研讨会 </a> <span> <span> . 2010</span> </span> </div> </li> <li> <div> <b>7. </b><a 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GUIDANCE AND PHOTOGRAPHIC CONDITION SETTING SERVICE SYSTEM</a> <b>[P]</b> . <span> 外国专利：  JP2002214681A </span> <span> . 2002-07-31</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：具有照相点引导功能和照相条件设置功能的照相机，以及照相点引导和照相条件设置服务系统 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130417737546.html">1. Explosive detonation system, including detonation device, including a bunker, a detonator, a rechargeable source, a shock tube, a shock tube explosive and a photoelectric chemical substance.</a> <b>[P]</b> . <span> 外国专利：  CL2013002402A1 </span> <span> . 2014-01-24</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：1.爆炸物爆炸系统，包括爆炸装置，其包括地堡，雷管，可再充电源，冲击管，冲击管炸药和光电化学物质。 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130441392457.html">Pressed insensitive explosive contains explosive crystals bound by binder system comprising a plasticizer and a composition containing a polyacrylic polymer</a> <b>[P]</b> . <span> 外国专利：  DE20220625U1 </span> <span> . 2003-12-24</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：压制的不敏感炸药包含由粘合剂体系粘合的炸药晶体，该粘合剂体系包含增塑剂和含有聚丙烯酸酯聚合物的组合物 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704024626639','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div class="journalsub-pop-up" style="display: none"> <div class="journal-sub"> <h2>期刊订阅</h2> <img src="https://cdn.zhangqiaokeyan.com/img/loginclose.png" alt="关闭" onclick="$('.journalsub-pop-up').hide()"> <p class="pardon">抱歉，该期刊暂不可订阅，敬请期待！</p> <p class="current">目前支持订阅全部北京大学中文核心（2020）期刊目录。</p> <div style="display: flex;margin-top: 69px;justify-content: 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