Formation of N‐Doped Carbon‐Coated ZnO/ZnCo <sub xmlns='http://www.wiley.com/namespaces/wiley'>2</sub>2 O <sub xmlns='http://www.wiley.com/namespaces/wiley'>4</sub>4 /CuCo <sub xmlns='http://www.wiley.com/namespaces/wiley'>2</sub>2 O <sub xmlns='http://www.wiley.com/namespaces/wiley'>4</sub>4 Derived from a Polymetallic Metal–Organic Framework: Toward High‐Rate and Long‐Cycle‐Life Lithium Storage

Niu Ji‐Liang; Zeng Cheng‐Hui; Peng Hai‐Jun; Lin Xiao‐Ming; Sathishkumar Palanivel; Cai Yue‐Peng

摘要

Abstract > Metal–organic frameworks (MOFs) are very promising self‐sacrificing templates for the large‐scale fabrication of new functional materials owing to their versatile functionalities and tunable porosities. Most conventional metal oxide electrodes derived from MOFs are limited by the low abundance of incorporated metal elements. This study reports a new strategy for the synthesis of multicomponent active metal oxides by the pyrolysis of polymetallic MOF precursors. A hollow N‐doped carbon‐coated ZnO/ZnCo <sub>2</sub> O <sub>4</sub> /CuCo <sub>2</sub> O <sub>4</sub> nanohybrid is prepared by the thermal annealing of a polymetallic MOF with ammonium bicarbonate as a pore‐forming agent. This is the first report on the rational design and preparation of a hybrid composed of three active metal oxide components originating from MOF precursors. Interestingly, as a lithium‐ion battery anode, the developed electrode delivers a reversible capacity of 1742 mAh g ?1 after 500 cycles at a current density of 0.3 mA g ?1 . Furthermore, the material shows large storage capacities (1009 and 667 mAh g ?1 ), even at high current flow (3 and 10 A g ?1 ). The remarkable high‐rate capability and outstanding long‐life cycling stability of the multidoped metal oxide benefits from the carbon‐coated integrated nanostructure with a hollow interior and the three active metal oxide components. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <title type =“main”>抽象</ title> >金属 - 有机框架（MOFS）非常有前途的自我牺牲模板，用于由于它们的多功能函数和可调孔隙率而大规模制造新的功能材料。衍生自MOF的大多数常规金属氧化物电极受到掺入金属元素的低丰度的限制。本研究报告了通过多金属MOF前体的热解的合成多组分活性金属氧化物的新策略。制备中空N-掺杂的碳涂覆的ZnO / ZnCo <sub> 2 </ sub> o <sub> 4 </ sub> o <sub> 4 </ sub>α1/ sum>纳米冬冬冬冬冬丙通过与碳酸氢铵作为孔形成剂的多金属MOF的热退火。这是第一份关于合理设计的报告，并由源自MOF前体的三种活性金属氧化物组分组成的杂种。有趣的是，作为锂离子电池阳极，在电流密度为0.3mA g 1 </ sup>的500次循环后，发达电极在500次循环之后，发达的电极可提供1742mahg Δ1</ sup>的可逆容量。此外，即使在高电流流动（3和10a g 1 </ sup>），该材料也显示了大的存储容量（1009和667mah g 1 </ sup> 1）。具有中空内部和三种活性金属氧化物组分的碳涂覆的集成纳米结构的碳涂覆的集成纳米结构的显着高速率能力和卓越的长寿命循环稳定性。 </ p> </ abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-28247/'>《Small》</a> <b style="margin: 0 2px;">|</b><span>2017年第47期</span><b style="margin: 0 2px;">|</b><span>共1页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Niu Ji‐Liang&option=202" target="_blank" rel="nofollow">Niu Ji‐Liang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zeng Cheng‐Hui&option=202" target="_blank" rel="nofollow">Zeng Cheng‐Hui;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Peng Hai‐Jun&option=202" target="_blank" rel="nofollow">Peng Hai‐Jun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lin Xiao‐Ming&option=202" target="_blank" rel="nofollow">Lin Xiao‐Ming;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Sathishkumar Palanivel&option=202" target="_blank" rel="nofollow">Sathishkumar Palanivel;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cai Yue‐Peng&option=202" target="_blank" rel="nofollow">Cai Yue‐Peng;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Guangzhou Key Laboratory of Materials for Energy Conversion and StorageSouth China Normal UniversityGuangzhou 510006 P. R. China;</p> <p>College of Chemistry and Chemical EngineeringJiangxi Normal UniversityNanchang 330022 P. R. China;</p> <p>Guangzhou Key Laboratory of Materials for Energy Conversion and StorageSouth China Normal UniversityGuangzhou 510006 P. R. China;</p> <p>Guangzhou Key Laboratory of Materials for Energy Conversion and StorageSouth China Normal UniversityGuangzhou 510006 P. R. China;</p> <p>Key Laboratory of Theoretical Chemistry of EnvironmentSouth China Normal UniversityGuangzhou 510006 P. R. China;</p> <p>Guangzhou Key Laboratory of Materials for Energy Conversion and StorageSouth China Normal UniversityGuangzhou 510006 P. R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=anode&option=203" rel="nofollow">anode;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hollow interior&option=203" rel="nofollow">hollow interior;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lithium storage&option=203" rel="nofollow">lithium storage;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanoparticles&option=203" rel="nofollow">nanoparticles;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=polymetallic metal–organic frameworks&option=203" rel="nofollow">polymetallic metal–organic frameworks;</a> </p> <div class="translation"> 机译：阳极;中空内部;锂储存;纳米粒子;多金属 - 有机框架; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704024267214.html">Formation of N‐Doped Carbon‐Coated ZnO/ZnCo <sub xmlns="http://www.wiley.com/namespaces/wiley">2</sub>2 O 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Formation of N‐Doped Carbon‐Coated ZnO/ZnCo 22 O 44 /CuCo 22 O 44 Derived from a Polymetallic Metal–Organic Framework: Toward High‐Rate and Long‐Cycle‐Life Lithium Storage

摘要

Formation of N‐Doped Carbon‐Coated ZnO/ZnCo ₂2 O ₄4 /CuCo ₂2 O ₄4 Derived from a Polymetallic Metal–Organic Framework: Toward High‐Rate and Long‐Cycle‐Life Lithium Storage