High‐Performance Aqueous Zinc–Ion Battery Based on Layered H <sub xmlns='http://www.wiley.com/namespaces/wiley'>2</sub>2 V <sub xmlns='http://www.wiley.com/namespaces/wiley'>3</sub>3 O <sub xmlns='http://www.wiley.com/namespaces/wiley'>8</sub>8 Nanowire Cathode

He Pan; Quan Yueli; Xu Xu; Yan Mengyu; Yang Wei; An Qinyou; He Liang; Mai Liqiang

摘要

Abstract > Rechargeable aqueous zinc–ion batteries have offered an alternative for large‐scale energy storage owing to their low cost and material abundance. However, developing suitable cathode materials with excellent performance remains great challenges, resulting from the high polarization of zinc ion. In this work, an aqueous zinc–ion battery is designed and constructed based on H <sub>2</sub> V <sub>3</sub> O <sub>8</sub> nanowire cathode, Zn(CF <sub>3</sub> SO <sub>3</sub> ) <sub>2</sub> aqueous electrolyte, and zinc anode, which exhibits the capacity of 423.8 mA h g ?1 at 0.1 A g ?1 , and excellent cycling stability with a capacity retention of 94.3% over 1000 cycles. The remarkable electrochemical performance is attributed to the layered structure of H <sub>2</sub> V <sub>3</sub> O <sub>8</sub> with large interlayer spacing, which enables the intercalation/de‐intercalation of zinc ions with a slight change of the structure. The results demonstrate that exploration of the materials with large interlayer spacing is an effective strategy for improving electrochemical stability of electrodes for aqueous Zn ion batteries. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <title type =“main”>抽象</ title> >可充电水由于其低成本和材料丰富，锌离子电池提供了大规模储能的替代方案。然而，开发具有优异性能的合适的阴极材料仍然存在巨大的挑战，由锌离子的高偏振产生。在这项工作中，基于H <sub> 2 </ sub> V <sub> 3 </ sub> O <sub> 8 </ sum>纳米线阴极，Zn（Cf <亚> 3 </ sup> SO <sub> 3 </ sub>）<sub> 2 </ sub>含水电解质和锌阳极，其能力为423.8 mA hg 1/pl 0.1 a g ？1 </ sup>，优异的循环稳定性，容量保留超过1000次循环。显着的电化学性能归因于H <sub> 2 </ sub> V <sub> 3 </ sub> O <sub> 8 </ sub>的分层结构，其具有大层间间距，这使得嵌入/ de-锌离子与结构略有变化的嵌入。结果表明，具有大层间间距的材料的探测是提高Zn离子电池水溶液电化学稳定性的有效策略。 </ p> </ abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" > 著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-28247/'>《Small 》</a> <b style="margin: 0 2px;">|</b><span>2017年第47期</span><b style="margin: 0 2px;">|</b> <span>共1页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=He Pan&option=202" target="_blank" rel="nofollow">He Pan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Quan Yueli&option=202" target="_blank" rel="nofollow">Quan Yueli;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Xu&option=202" target="_blank" rel="nofollow">Xu Xu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yan Mengyu&option=202" target="_blank" rel="nofollow">Yan Mengyu;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yang Wei&option=202" target="_blank" rel="nofollow">Yang Wei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=An Qinyou&option=202" target="_blank" rel="nofollow">An Qinyou;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=He Liang&option=202" target="_blank" rel="nofollow">He Liang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Mai Liqiang&option=202" target="_blank" rel="nofollow">Mai Liqiang;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>State Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of TechnologyWuhan 430070 P. R. China;</p> <p>State Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of TechnologyWuhan 430070 P. R. China;</p> <p>State Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of TechnologyWuhan 430070 P. R. China;</p> <p>State Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of TechnologyWuhan 430070 P. R. China;</p> <p>State Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of TechnologyWuhan 430070 P. R. China;</p> <p>State Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of TechnologyWuhan 430070 P. R. China;</p> <p>State Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of TechnologyWuhan 430070 P. R. China;</p> <p>State Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of TechnologyWuhan 430070 P. R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li> <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span> <a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料 ;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=H 2 V 3 O 8&option=203" rel="nofollow">H 2 V 3 O 8;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=intercalation reaction&option=203" rel="nofollow">intercalation reaction;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=large‐scale energy storage&option=203" rel="nofollow">large‐scale energy storage;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=zinc–ion batteries&option=203" rel="nofollow">zinc–ion batteries;</a> </p> <div class="translation"> 机译：H 2 V 3 O 8;嵌入反应;大规模储能;锌离子电池; 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High‐Performance Aqueous Zinc–Ion Battery Based on Layered H 22 V 33 O 88 Nanowire Cathode

摘要

High‐Performance Aqueous Zinc–Ion Battery Based on Layered H ₂2 V ₃3 O ₈8 Nanowire Cathode