The sensitivity of capacitive pressure sensors is primarily determined by themodulus of a soft dielectric layer that reversibly deforms to produce an electrical signal. Unfortunately, the mechanical properties of conventional linear networks are constrained such that a lower limit on softness translates to poor capacitive pressure sensor performance. Here, we overcome this paradigm by leveraging the intrinsic "supersoft'' characteristic of bottlebrush polymers. A simple light-induced crosslinking strategy is introduced to facilitate device fabrication and parallel plate capacitive pressure sensors constructed with these bottlebrush polymer networks exhibit up to a 53x increase in sensitivity compared to traditional material formulations, e.g., Sylgard 184. This combination of contemporary synthetic chemistry and application-driven materials design accentuates the opportunities available at the intersection of science and engineering.
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