Development of 1 kW‐class Ammonia‐fueled Solid Oxide Fuel Cell Stack

摘要

Abstract > Power generation performance and long‐term durability of ammonia‐fueled solid oxide fuel cell (SOFC) systems are investigated with SOFC stacks consisting of 30 planar anode‐supported cells. SOFC systems with three different operation modes are employed: direct ammonia, external decomposition and autothermal decomposition. A novel BaO/Ni/Sm <sub>2</sub> O <sub>3</sub> /MgO catalyst is newly developed for the external ammonia cracker, whereas a Co‐Ce‐Zr composite oxide catalyst is used for the autothermal ammonia cracker. Initial performance measurement and 1,000?h long‐term durability test of the stacks are conducted. The stack fueled with direct ammonia achieves 1?kW power output with 52% direct current (DC) electrical efficiency; a slight decrease in its performance compared with the stack with the mixture fuel of hydrogen and nitrogen is attributed to the decrease in the stack temperature caused by the endothermic ammonia decomposition reaction. The external ammonia cracker helps to maintain the stack temperature, improving the initial performance of the stack. The stack performance with the autothermal ammonia cracker is also comparable to those with the other operation modes. It is also demonstrated that the stacks fueled with ammonia have excellent stability during the long‐term tests and 57% energy conversion efficiency at ca.?700?W electrical output is achieved with the external ammonia cracker. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 用由30个平面阳极支持的细胞组成的SOFC叠层研究了氨燃料固体氧化物燃料电池（SOFC）系统的发电性能和长期耐久性。采用具有三种不同操作模式的SOFC系统：直接氨，外部分解和自热分解。一个新的bao / ni / sm <sub> 2 </ sub> O. <sub> 3 </ sub> / MgO催化剂是用于外部氨裂化器的新开发的，而CO-CE-ZR复合氧化物催化剂用于自热氨裂解器。进行初始性能测量和堆叠的长期耐久性测试。用直接氨燃料的堆叠实现了1？KW功率输出，直流电流（直流）电效率为52％;与具有氢气和氮气的混合物燃料的堆叠相比，其性能的略微降低归因于吸热氨分解反应引起的堆叠温度的降低。外部氨饼干有助于保持堆叠温度，提高堆叠的初始性能。具有自动氨氨饼干的堆叠性能也与具有其他操作模式的堆叠性能相当。还证明，在长期测试期间，用氨燃料的堆叠具有出色的稳定性，并且在CA.?700OWOWOWOWOWEL输出中实现了57％的能量转换效率。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-24199/'>《Fuel cells》</a> <b style="margin: 0 2px;">|</b><span>2020年第1期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1817.html" title="电化学工业">电化学工业;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ammonia&option=203" rel="nofollow">Ammonia;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Catalyst&option=203" rel="nofollow">Catalyst;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Durability&option=203" rel="nofollow">Durability;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Solid Oxide Fuel Cell&option=203" rel="nofollow">Solid Oxide Fuel Cell;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Stack&option=203" rel="nofollow">Stack;</a> </p> <div class="translation"> 机译：氨;催化剂;耐久性;固体氧化物燃料电池;堆叠; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704023515297.html">Development of 1 kW‐class Ammonia‐fueled Solid Oxide Fuel Cell Stack</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> </a> <a href="/journal-foreign-24199/" target="_blank" rel="nofollow" class="tuijian_authcolor">Fuel cells .</a> <span>2020</span><span>,第1期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：开发1千瓦级氨燃料固体氧化物燃料电池堆</span> </p> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/academic-journal-foreign_journal-power-sources_thesis/020416274510.html">Development Of 1 Kw Class Solid Oxide Fuel Cell Stack Using Anode-supported Planar Cells</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=M. 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class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020314279792.html">质子交换膜燃料电池数学模型及千瓦级电堆的实验研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=胡鸣若&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 胡鸣若</a> <span> . 2004</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061204387014.html">一种固体氧化物燃料电池堆、基于该固体氧化物燃料电池堆的无人机增程控制系统及方法</a> <b>[P]</b> . <span> 中国专利： CN111162303B </span> <span> . 2021.05.07</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120103812430.html">一种固体氧化物燃料电池堆、基于该固体氧化物燃料电池堆的无人机增程控制系统及方法</a> <b>[P]</b> . <span> 中国专利： CN111162303A </span> <span> . 2020-05-15</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130426520998.html">SOLID ELECTROLYTE FUEL CELL COMPOSITE OXIDE, SOLID ELECTROLYTE FUEL CELL BINDER, SOLID ELECTROLYTE FUEL CELL ELECTRODE, SOLID ELECTROLYTE FUEL CELL COLLECTOR MEMBER, SOLID ELECTROLYTE FUEL CELL, SOLID ELECTROLYTE FUEL CELL STACK, AND MANUFACTURING METHOD OF SOLID ELECTROLYTE FUEL CELL COMPOSITE OXIDE MIXTURE</a> <b>[P]</b> . <span> 外国专利：  JP2011228009A </span> <span> . 2011-11-10</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：固体电解质燃料电池复合氧化物，固体电解质燃料电池粘合剂，固体电解质燃料电池电极，固体电解质燃料电池集电极，固体电解质燃料电池，固体电解质和固体电解质 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130435922018.html">SOLID OXIDE FUEL CELL STACK, SOLID OXIDE FUEL CELL MODULE USING THIS, AND MANUFACTURING METHOD OF SOLID OXIDE FUEL CELL STACK</a> <b>[P]</b> . <span> 外国专利：  JP2006351253A </span> <span> . 2006-12-28</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：固体氧化物燃料电池堆，使用该固体氧化物燃料电池堆的模块以及固体氧化物燃料电池堆的制造方法 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130415193717.html">Method for operating a variable energy output solid oxide fuel cell stack, control system for a variable energy output solid oxide fuel cell stack, and a mixed ion / electron conducting electrolyte fuel cell stack.</a> <b>[P]</b> . <span> 外国专利：  BRPI0507602B1 </span> <span> . 2015-08-04</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：用于操作可变能量输出固体氧化物燃料电池堆的方法，用于可变能量输出固体氧化物燃料电池堆的控制系统以及混合的离子/电子传导电解质燃料电池堆。 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img 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