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首页> 外文期刊>Fuel cells >Layer‐by‐layer Proton Donor and Acceptor Membrane for an Efficient Proton Transfer System in a Polymer Electrolyte Membrane Fuel Cell
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Layer‐by‐layer Proton Donor and Acceptor Membrane for an Efficient Proton Transfer System in a Polymer Electrolyte Membrane Fuel Cell

机译：用于高分子电解质膜燃料电池中有效质子转移系统的逐层质子供体和受体膜

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Abstract >The high performance proton transfer in polymer electrolyte membranes (PEMs) is known to be achieved through cooperating of proton donors and acceptors. In order to obtain the effective and efficient proton transfer, the present work proposes a membrane with proton donors and proton acceptors in layer‐by‐layer (LbL) structure. By applying sulfonated poly (ether ether ketone) (SPEEK) as the substrate membrane and soaking alternatively with the proton donor polymer, i.e. poly(acrylic acid) (PAA), and the proton acceptor heterocycles, i.e. benzimidazoles (BI), the LbL SPEEK/BI/PAA membranes can be achieved. The systematic variation based on the branching benzimidazole groups suggest that the LbL SPEEK/BI/PAA membrane obtained shows an increase in proton conductivity compared to the neat SPEEK, especially in the case of the membrane with trifunctional benzimidazole (B4) is as high as 1–2.5 orders of magnitude over the temperature range of 30–170?°C. The present work points out the simple surface modification of the proton conductive membrane by layer‐by‐layer approach as a practical and simple way to enhance the performance of polymer electrolyte membrane. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract XMLNS =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <标题类型=“main”>抽象</ title> 已知通过配合质子供体和受体来实现聚合物电解质膜（PEMS）中的高性能质子转移。为了获得有效和有效的质子转移，本作者提出了一种具有质子供体的膜和逐层（LBL）结构的质子受体。通过将磺化聚（醚醚酮）（Speek）作为底物膜施用，也可以浸泡质子供体聚合物，即聚（丙烯酸）（PAA），以及质子受体杂环，即苯并咪唑（BI），LBL Speek / BI / PAA膜可以实现。基于支化苯并咪唑基团的系统变化表明，与整洁的苯甲基菜相比，所获得的LBL Speek / Bi / Paa膜显示出质子电导率的增加，特别是在具有三官能苯并咪唑（B4）的膜的情况下高达1 -2.5在30-170°C的温度范围内的数量级。本工作指出了通过层逐方法作为一种实用而简单的方法来提高聚合物电解质膜的性能的实用而简单的表面改性。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-24199/'>《Fuel cells》</a> <b style="margin: 0 2px;">|</b><span>2018年第2期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Meemuk C.&option=202" target="_blank" rel="nofollow">Meemuk C.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Chirachanchai S.&option=202" target="_blank" rel="nofollow">Chirachanchai S.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>The Petroleum and Petrochemical CollegeChulalongkorn UniversityBangkok Thailand;</p> <p>The Petroleum and Petrochemical CollegeChulalongkorn UniversityBangkok Thailand;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1817.html" title="电化学工业">电化学工业;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Benzimidazole&option=203" rel="nofollow">Benzimidazole;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Poly(acrylic acid)&option=203" rel="nofollow">Poly(acrylic acid);</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Polymer Electrolyte Membrane Fuel Cell&option=203" rel="nofollow">Polymer Electrolyte Membrane Fuel Cell;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Proton Acceptor&option=203" rel="nofollow">Proton Acceptor;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Proton Donor&option=203" rel="nofollow">Proton Donor;</a> </p> <div class="translation"> 机译：苯并咪唑;聚（丙烯酸）;聚合物电解质膜燃料电池;质子受体;质子供体; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div 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href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=栾辉宝&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,栾辉宝</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=陶文铨&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,陶文铨</a> <span> <a href="/conference-cn-10569/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 2011年中国工程热物理学会传热传质学学术会议 </a> <span> <span> . 2011</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020315692092.html">高温质子交换膜燃料电池用新型质子膜和气体扩散层构筑及性能研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=李涛&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 李涛</a> <span> . 2020</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/06120108619127.html">高分子电解质组合物、以及使用其的高分子电解质膜、被覆催化剂层的电解质膜、膜电极复合体及固体高分子型燃料电池</a> <b>[P]</b> . <span> 中国专利： CN106133976A </span> <span> . 2016-11-16</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120105624040.html">燃料电池用电解质膜用多孔材料、其制造方法、固体高分子型燃料电池用电解质膜、膜－电极接合体(MEA)、和燃料电池</a> <b>[P]</b> . <span> 中国专利： CN101421876A </span> <span> . 2009-04-29</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130418537846.html">Proton conductive material, proton conductive electrolyte membrane, proton conductive electrolyte membrane with proton conductive electrolyte layer, membrane-electrode assembly, and polymer electrolyte fuel cell</a> <b>[P]</b> . <span> 外国专利： <!-- 日本专利： --> JP5480578B2 </span> <span> . 2014-04-23</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：质子传导性材料，质子传导性电解质膜，具有质子传导性电解质层的质子传导性电解质膜，膜电极接合体以及高分子电解质燃料电池 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130426440607.html">PROTON CONDUCTIVE MATERIAL, PROTON CONDUCTIVE ELECTROLYTE MEMBRANE, PROTON CONDUCTIVE ELECTROLYTE MEMBRANE WITH PROTON CONDUCTIVE ELECTROLYTE LAYER, MEMBRANE-ELECTRODE ASSEMBLY, AND POLYMER ELECTROLYTE FUEL CELL</a> <b>[P]</b> . <span> 外国专利： <!-- 日本专利： --> JP2011074196A </span> <span> . 2011-04-14</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：质子传导性材料，质子传导性电解质膜，质子传导性电解质层的质子传导性电解质膜，膜电极组装体以及高分子电解质燃料电池 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130405442213.html">POLYPHENYLSULFONE-BASED PROTON CONDUCTING POLYMER ELECTROLYTE, PROTON CONDUCTING SOLID POLYMER ELECTROLYTE MEMBRANE, ELECTRODE CATALYST LAYER FOR SOLID POLYMER FUEL CELLS, METHOD FOR PRODUCING ELECTRODE CATALYST LAYER FOR SOLID POLYMER FUEL CELLS, AND FUEL CELL</a> <b>[P]</b> . <span> 外国专利： <!-- 欧洲知识产权局专利： --> EP3340350A4 </span> <span> . 2019-04-17</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：聚苯砜基质子传导聚合物电解质，质子传导固体聚合物电解质膜，用于固体聚合物燃料电池的电极催化剂层，用于制造电极催化剂的溶液，用于固体聚合物的电解质溶液 </span> </p> </li> </ul> </div> </div> </div> <div class="theme cardcommon" style="overflow: auto;display:none"> <h3 class="all_title" id="enpatent55">相关主题</h3> <ul id="subject"> </ul> </div> </div> </div> </div> <div class="right rightcon"> <div class="details_img cardcommon clearfix" style="margin-bottom: 10px;display:none;" > </div> </div> </div> <div id="thesis_get_original1" class="downloadBth" style="bottom: 19px;z-index: 999;" onclick="ywcd('0704023515172','4',7,2,1,'',this,24)" class="delivery" prompt="010401" title="通过人工服务将文献原文发送至邮箱" >获取原文</div> <div 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