In Situ Growth of Cobalt Nanoparticles Encapsulated Nitrogen‐Doped Carbon Nanotubes among Ti        <sub >3</sub>3        C        <sub >2</sub>2        T        <i >          <sub>x</sub>                  <sub >x</sub>x                (MXene) Matrix for Oxygen Reduction and Evolution

Zhang Youkui; Jiang Hongliang; Lin Yunxiang; Liu Hengjie; He Qun; Wu Chuanqiang; Duan Tao; Song Li

摘要

Abstract > MXene with unique layered structure and rich chemical compositions has been extensively investigated for lithium‐ion batteries, electrochemical capacitors, and hydrogen storage medium, but less attention has been paid to its electrocatalytic potential might due to nonideal activity. Here, an in situ growth strategy is developed to synthesize a new type of composite with carbon nanotubes (CNTs) supported on the surface of Ti <sub>3</sub> C <sub>2</sub> T <sub>x</sub> MXene (Co/N‐CNTs@Ti <sub>3</sub> C <sub>2</sub> T <sub>x</sub> ) as bifunctional electrocatalyst toward oxygen reduction reaction (ORR) and oxygen evolution reaction (OER). By combining the X‐ray photoelectron detection with synchrotron‐based soft X‐ray spectroscopic characterizations, the strong interfacial coupling and electron transfer are efficiently identified, which can effectively facilitate the bifunctional electrocatalytic performance of Co/N‐CNTs@Ti <sub>3</sub> C <sub>2</sub> T <sub>x</sub> toward ORR and OER in alkaline solution. The present strategy provides a facile route for the design of the hybrids of CNTs and MXene for bifunctional electrocatalysis. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 对于锂离子电池，电化学电容器和储氢介质，具有独特的层状结构和富含化学成分的蒙片，而且对其电催化可能导致的锂离子电池，电化学电容和储氢介质具有较少的注意力。在这里，开发了一种原位生长策略，以将新型的复合材料用TI表面支撑的碳纳米管（CNT）合成 <sub> 3 </ sub> C <sub> 2 </ sub> T. <sub> x </ sub> </ i> MXENE（CO / N-CNTS @ TI <sub> 3 </ sub> C <sub> 2 </ sub> T. <sub> x </ sub> </ i> ）作为双功能性电催化剂朝向氧还原反应（ORR）和氧气进化反应（OER）。通过将X射线光电子检测与基于同步的软X射线光谱特征相结合，有效地识别出强的界面耦合和电子传递，可以有效地促进CNT的双功能电催化性能@ TI <sub> 3 </ sub> C <sub> 2 </ sub> T. <sub> x </ sub> </ i> 朝向碱性解决方案的ORR和OER。本策略提供了用于设计CNT和MXENE用于双官能电常见的杂种的容易途径。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第16期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Youkui&option=202" target="_blank" rel="nofollow">Zhang Youkui;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jiang Hongliang&option=202" target="_blank" rel="nofollow">Jiang Hongliang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lin Yunxiang&option=202" target="_blank" rel="nofollow">Lin Yunxiang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Hengjie&option=202" target="_blank" rel="nofollow">Liu Hengjie;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=He Qun&option=202" target="_blank" rel="nofollow">He Qun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wu Chuanqiang&option=202" target="_blank" rel="nofollow">Wu Chuanqiang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Duan Tao&option=202" target="_blank" rel="nofollow">Duan Tao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Song Li&option=202" target="_blank" rel="nofollow">Song Li;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>National Synchrotron Radiation LaboratoryUniversity of Science and Technology of ChinaHefei 230029 China;</p> <p>National Synchrotron Radiation LaboratoryUniversity of Science and Technology of ChinaHefei 230029 China;</p> <p>National Synchrotron Radiation LaboratoryUniversity of Science and Technology of ChinaHefei 230029 China;</p> <p>National Synchrotron Radiation LaboratoryUniversity of Science and Technology of ChinaHefei 230029 China;</p> <p>National Synchrotron Radiation LaboratoryUniversity of Science and Technology of ChinaHefei 230029 China;</p> <p>National Synchrotron Radiation LaboratoryUniversity of Science and Technology of ChinaHefei 230029 China;</p> <p>School of National Defense Science and TechnologySouthwest University of Science and TechnologyMianyang 621010 China;</p> <p>National Synchrotron Radiation LaboratoryUniversity of Science and Technology of ChinaHefei 230029 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=carbon nanotubes&option=203" rel="nofollow">carbon nanotubes;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=MXene&option=203" rel="nofollow">MXene;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=oxygen reduction and evolution&option=203" rel="nofollow">oxygen reduction and evolution;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=X‐ray absorption spectra&option=203" rel="nofollow">X‐ray absorption spectra;</a> </p> <div class="translation"> 机译：碳纳米管;MXENE;氧气还原和进化;X射线吸收光谱; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022435627.html">In Situ Growth of Cobalt Nanoparticles Encapsulated Nitrogen‐Doped Carbon Nanotubes among Ti <sub >3</sub>3 C <sub >2</sub>2 T <i > <sub>x</sub> <sub >x</sub>x (MXene) Matrix for Oxygen Reduction and Evolution</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Youkui&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Zhang Youkui,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jiang 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nanotubes encapsulated particles of nickel and cobalt and plants for the synthesis of materials based on carbon nanotubes and nanoparticles of nickel or cobalt</a> <b>[P]</b> . <span> 外国专利：  RU2005132267A </span> <span> . 2007-04-27</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：碳纳米管封装的镍和钴纳米粒子的制备方法以及用于合成基于碳纳米管和镍或钴纳米粒子的材料的植物 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130417861599.html">Nitrogen-doped carbon-supported cobalt-iron oxygen reduction catalyst</a> <b>[P]</b> . <span> 外国专利：  US8709295B2 </span> <span> . 2014-04-29</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：氮掺杂碳载钴铁氧还原催化剂 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" 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In Situ Growth of Cobalt Nanoparticles Encapsulated Nitrogen‐Doped Carbon Nanotubes among Ti 33 C 22 T x xx (MXene) Matrix for Oxygen Reduction and Evolution

摘要

In Situ Growth of Cobalt Nanoparticles Encapsulated Nitrogen‐Doped Carbon Nanotubes among Ti ₃3 C ₂2 T _x _xx (MXene) Matrix for Oxygen Reduction and Evolution