Co‐Modified MoS        <sub >2</sub>2        Hybrids as Superior Bifunctional Electrocatalysts for Water Splitting Reactions: Integrating Multiple Active Components in One

Zhao Zhong‐Yin; Li Fei‐Long; Shao Qi; Huang Xiaoqing; Lang Jian‐Ping

摘要

Abstract > The development of highly active, stable, low‐cost, and earth‐abundant electrocatalysts for both hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) remains a great challenge. Herein, the cobalt (Co)‐modified MoS <sub>2</sub> hybrid catalysts grown on nickel foam (NF) are successfully synthesized by a facile solvothermal method. The optimized catalyst (denoted as Co‐Mo‐S‐2/NF) shows excellent HER activity with low overpotentials of 77 and 96 mV at a current density of 10 mA cm ?2 , as well as excellent stability with negligible loss of the cathodic current after 3000 cycles in 1.0 M KOH and 1.0 M phosphate‐buffered saline (pH = 7), respectively. Significantly, when used as OER catalyst, the Co‐Mo‐S‐2/NF hybrid also displays outstanding OER activity with a low overpotential of 294 mV at a current density of 10 mA cm ?2 and good long‐term stability for 120 h at 10 mA cm ?2 without observable fading under alkaline condition. The excellent electrocatalytic activity of the generated catalyst is mainly due to abundant active site, large active area, improved conductivity, and synergistic effect within MoS <sub>2</sub> , Co <sub>9</sub> S <sub>8</sub> , and CoMoS <sub>3.13</sub> . This work provides a unique strategy to design the high‐performance and stable electrocatalysts for HER and OER. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 对于氢气进化反应（她）和氧气进化反应（Oer）的高活性，稳定，低成本和地球丰富的电催化剂的发展仍然是一个很大的挑战。在此，钴（CO）制定的MOS <sub> 2 </ sub> 在镍泡沫（NF）上生长的杂化催化剂通过容易的溶剂热法成功地合成。优化的催化剂（表示为CO-MO-S-2 / NF）显示出优异的优异活性，其活性为77和96mV，电流密度为10 mA cm ？2 </ sup> 尽管在1.0M KOH和1.0M磷酸盐缓冲盐水（pH = 7）中，但在1.0M KOH和1.0M磷酸盐缓冲盐水（pH = 7）中，具有优异的稳定性。显着，当用作OER催化剂时，CO-MO-S-2 / NF混合动力车还显示出具有294mV的低过电位的优异的OER活动，其电流密度为10 mA cm ？2 </ sup> 良好的长期稳定性120小时，10 ma cm ？2 </ sup> 在碱性条件下没有明显的褪色。所产生的催化剂的优异电催化活性主要是由于富有的活性位点，大量的有源区，改善的导电性和在MOS内的协同作用。 <sub> 2 </ sub> ，CO. <sub> 9 </ sub> S. <sub> 8 </ sub> 和comos. <sub> 3.13 </ sub> 。这项工作提供了独特的策略，可以为她和Oer设计高性能和稳定的电催化剂。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2019年第11期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhao Zhong‐Yin&option=202" target="_blank" rel="nofollow">Zhao Zhong‐Yin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Fei‐Long&option=202" target="_blank" rel="nofollow">Li Fei‐Long;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Shao Qi&option=202" target="_blank" rel="nofollow">Shao Qi;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang Xiaoqing&option=202" target="_blank" rel="nofollow">Huang Xiaoqing;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lang Jian‐Ping&option=202" target="_blank" rel="nofollow">Lang Jian‐Ping;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>College of ChemistrySoochow UniversityJiangsu 215123 China;</p> <p>College of ChemistrySoochow UniversityJiangsu 215123 China;</p> <p>College of ChemistrySoochow UniversityJiangsu 215123 China;</p> <p>College of ChemistrySoochow UniversityJiangsu 215123 China;</p> <p>College of ChemistrySoochow UniversityJiangsu 215123 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Co‐modified MoS 2 hybrid&option=203" rel="nofollow">Co‐modified MoS 2 hybrid;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrocatalyst&option=203" rel="nofollow">electrocatalyst;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hydrogen evolution reaction&option=203" rel="nofollow">hydrogen evolution reaction;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=oxygen evolution reaction&option=203" rel="nofollow">oxygen evolution reaction;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=synergistic effect&option=203" rel="nofollow">synergistic effect;</a> </p> <div class="translation"> 机译：共改性MOS 2杂交;电催化剂;氢气进化反应;氧气进化反应;协同效应; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022434986.html">Co‐Modified MoS <sub >2</sub>2 Hybrids as Superior Bifunctional Electrocatalysts for Water Splitting Reactions: Integrating Multiple Active Components in One</a> 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Co‐Modified MoS 22 Hybrids as Superior Bifunctional Electrocatalysts for Water Splitting Reactions: Integrating Multiple Active Components in One

摘要

Co‐Modified MoS ₂2 Hybrids as Superior Bifunctional Electrocatalysts for Water Splitting Reactions: Integrating Multiple Active Components in One