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Lubricin Antiadhesive Coatings Exhibit Size‐Selective Transport Properties that Inhibit Biofouling of Electrode Surfaces with Minimal Loss in Electrochemical Activity

机译：润滑油抗结构涂层表现出尺寸选择性的运输性能，抑制电极表面的生物污染，电化学活性损失最小

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Abstract > Electrochemical sensing is a highly effective technique for rapidly detecting and quantifying the presence of electroactive compounds in solution. However, effective sensing requires the electrode surface to be free of contamination, which makes this technique particularly susceptible to the effects of surface fouling due to the unwanted adhesion of biomolecules. Unfortunately, coating electrodes with antiadhesive molecules typically causes electrical passivation with detrimental effects upon electrochemical processes. Lubricin is a large glycoprotein found in articular joints, which self‐assembles on most substrates and exhibits excellent antiadhesive properties. This report finds that lubricin antiadhesive coatings function as a size‐selective transport barrier that physically blocks large, fouling molecules (e.g., proteins) while still allowing small molecules to diffuse into, out‐of, and within this layer more‐or‐less unimpeded. The diffuse nature of the lubricin coatings ensures the electrode retains a large, “free” surface area that facilitates efficient charge transfer. Using cyclic voltammetry to measure the oxidation/reduction of a K <sub>3</sub> [Fe(CN) <sub>6</sub> ] redox couple at a gold electrode (a system particularly susceptible to fouling), this report shows that antiadhesive lubricin brush coatings can be used for highly sensitive amperometric/voltametric detection of small electroactive compounds in highly fouling solutions of proteins and blood plasma with minimal, immediate impact upon the electrochemistry. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 电化学感测是一种高效的技术，用于快速检测和定量溶液中电活性化合物的存在。然而，有效的感测要求电极表面没有污染，这使得这种技术由于生物分子的不希望的粘附而特别易于表面污垢的影响。遗憾的是，具有抗粘附分子的涂布电极通常会对电化学方法的有害影响导致电钝化。润滑油是在关节关节中发现的大糖蛋白，其在大多数底物上自组装并表现出优异的抗粘附性。本报告发现润滑素抗粘附涂层用作尺寸选择性的运输屏障，其在仍然允许小分子仍然弥漫于，在该层中延伸，并且在该层中仍然不受阻碍地延伸到大型，污垢分子（例如，蛋白质）的尺寸选择性运输屏障。。润滑油涂层的漫射性质确保电极保留了有助于有效电荷转移的大型“自由”表面积。使用循环伏安法测量k的氧化/减少 <sub> 3 </ sub> [Fe（CN） <sub> 6 </ sub> ]氧化还原耦合在金电极（一个特别容易受到污垢的系统），本报告显示，抗粘附性润滑油刷涂层可用于高敏感的电流/伏特检测小电活性化合物，以极少的蛋白质和血浆的溶液和血浆的高污垢溶液。立即影响电化学。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第7期</span><b style="margin: 0 2px;">|</b><span>共10页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Greene George W.&option=202" target="_blank" rel="nofollow">Greene George W.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ortiz Vanessa&option=202" target="_blank" rel="nofollow">Ortiz Vanessa;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Pozo‐Gonzalo Cristina&option=202" target="_blank" rel="nofollow">Pozo‐Gonzalo Cristina;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Moulton Simon E.&option=202" target="_blank" rel="nofollow">Moulton Simon E.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Xiaoen&option=202" target="_blank" rel="nofollow">Wang Xiaoen;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Martin Lisandra L.&option=202" target="_blank" rel="nofollow">Martin Lisandra L.;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Michalczky Agnes&option=202" target="_blank" rel="nofollow">Michalczky Agnes;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Howlett Patrick C.&option=202" target="_blank" rel="nofollow">Howlett Patrick C.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Institute for Frontier Materials and ARC Centre of Excellence for Electromaterials ScienceDeakin University75 Pigdons Road Geelong VIC 3216 Australia;</p> <p>Institut Charles Gerhardt MontpellierUniversité MontpellierPlace E. Bataillon 34 095 Montpellier France;</p> <p>Institute for Frontier Materials and ARC Centre of Excellence for Electromaterials ScienceDeakin University75 Pigdons Road Geelong VIC 3216 Australia;</p> <p>School of Software and Electrical Engineering and Department of TelecommunicationsSwinburne UniversityJohn St Hawthorn VIC 3122 Australia;</p> <p>Institute for Frontier Materials and ARC Centre of Excellence for Electromaterials ScienceDeakin University75 Pigdons Road Geelong VIC 3216 Australia;</p> <p>School of ChemistryMonash UniversityWellington Rd Clayton 3800 Australia;</p> <p>School of Life and Environmental ScienceDeakin University221 Burwood Highway Burwood 3125 Australia;</p> <p>Institute for Frontier Materials and ARC Centre of Excellence for Electromaterials ScienceDeakin University75 Pigdons Road Geelong VIC 3216 Australia;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=antiadhesive&option=203" rel="nofollow">antiadhesive;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=biosensors&option=203" rel="nofollow">biosensors;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=coatings&option=203" rel="nofollow">coatings;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrochemistry&option=203" rel="nofollow">electrochemistry;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lubricin&option=203" rel="nofollow">lubricin;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=permselectivity&option=203" rel="nofollow">permselectivity;</a> </p> <div class="translation"> 机译：抗粘附剂;生物传感器;涂料;电化学;润滑油;合格选择性; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022434739.html">Anti‐Adhesive Coatings: Lubricin Antiadhesive Coatings Exhibit Size‐Selective Transport Properties that Inhibit Biofouling of Electrode Surfaces with Minimal Loss in Electrochemical Activity (Adv. 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