Facile Synthesis of Nitrogen and Halogen Dual‐Doped Porous Graphene as an Advanced Performance Anode for Lithium‐Ion Batteries

Liu Huanlong; Tang Yufeng; Zhao Wei; Ding Wei; Xu Jijian; Liang Chenliang; Zhang Zhichao; Lin Tianquan; Huang Fuqiang

摘要

Abstract > Nonmetal‐dual doped graphene has attracted considerable attention as high‐performance anode material for lithium‐ion batteries (LIBs) due to the synergistic effects of heteroatom dopants. Herein, nitrogen and halogen (including Cl, Br, and I) dual‐doped graphene is successfully synthesized by a general wet chemical method and lithium storage performance of N, Cl codoped graphene as anode material for LIBs is investigated in detail. The dual‐doped heteroatoms introduce abundant defects and expand the interlayer spacing of graphene to benefit lithium insertion and extraction. When used as a typical anode material, the N and Cl dual‐doped porous graphene reveals a high specific capacity of 1200 mA h g ?1 at 0.1 A g ?1 and 1010 mA h g ?1 at 1.0 A g ?1 . The as‐prepared sample exhibits superior cycling performance, whose specific capacity remains 95% at 5.0 A g ?1 after 1800 cycles. The excellent performance mainly stems from the synergistic effect of structure modification and heteroatom doping, and the capacitive effects are dictated by kinetical analysis. The synthesized nitrogen and halogen dual‐doped porous graphene is a promising anode material for LIBs. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 由于杂原子掺杂剂的协同作用，非金属 - 双掺杂石墨烯吸引了锂离子电池（LIBS）的高性能阳极材料。本文，通过一般的湿化学方法和N，Cl Compoped石墨烯的锂储存性能成功地合成了双掺杂石墨烯，作为Libs的阳极材料，通过N，Cl Clopeed石墨烯的锂储存性能。双掺杂的杂原子引入了丰富的缺陷，并扩大了石墨烯的层间间距，使锂插入和提取。当用作典型的阳极材料时，N和Cl双掺杂多孔石墨烯显示出1200 mA H G的高比容量？1 </ sup> 在0.1克？1 </ sup> 和1010 ma h g ？1 </ sup> 在1.0克？1 </ sup> 。制备的样品具有优异的循环性能，其特定容量保持在5.0 A的95％？1 </ sup> 1800年后。优异的性能主要源于结构改性和杂原子掺杂的协同效应，并且电容效应由运动分析决定。合成的氮气和卤素双掺杂多孔石墨烯是Libs的有望的阳极材料。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-18063/'>《Advanced materials interfaces》</a> <b style="margin: 0 2px;">|</b><span>2018年第5期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Huanlong&option=202" target="_blank" rel="nofollow">Liu Huanlong;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tang Yufeng&option=202" target="_blank" rel="nofollow">Tang Yufeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhao Wei&option=202" target="_blank" rel="nofollow">Zhao Wei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ding Wei&option=202" target="_blank" rel="nofollow">Ding Wei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Jijian&option=202" target="_blank" rel="nofollow">Xu Jijian;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liang Chenliang&option=202" target="_blank" rel="nofollow">Liang Chenliang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Zhichao&option=202" target="_blank" rel="nofollow">Zhang Zhichao;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lin Tianquan&option=202" target="_blank" rel="nofollow">Lin Tianquan;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Huang Fuqiang&option=202" target="_blank" rel="nofollow">Huang Fuqiang;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>State Key Laboratory of High Performance Ceramics and Superfine MicrostructureChinese Academy of Sciences1295 Dingxi Road Shanghai 200050 China;</p> <p>State Key Laboratory of High Performance Ceramics and Superfine MicrostructureChinese Academy of Sciences1295 Dingxi Road Shanghai 200050 China;</p> <p>State Key Laboratory of High Performance Ceramics and Superfine MicrostructureChinese Academy of Sciences1295 Dingxi Road Shanghai 200050 China;</p> <p>State Key Laboratory of High Performance Ceramics and Superfine MicrostructureChinese Academy of Sciences1295 Dingxi Road Shanghai 200050 China;</p> <p>State Key Laboratory of High Performance Ceramics and Superfine MicrostructureChinese Academy of Sciences1295 Dingxi Road Shanghai 200050 China;</p> <p>State Key Laboratory of High Performance Ceramics and Superfine MicrostructureChinese Academy of Sciences1295 Dingxi Road Shanghai 200050 China;</p> <p>State Key Laboratory of High Performance Ceramics and Superfine MicrostructureChinese Academy of Sciences1295 Dingxi Road Shanghai 200050 China;</p> <p>State Key Laboratory of High Performance Ceramics and Superfine MicrostructureChinese Academy of Sciences1295 Dingxi Road Shanghai 200050 China;</p> <p>State Key Laboratory of High Performance Ceramics and Superfine MicrostructureChinese Academy of Sciences1295 Dingxi Road Shanghai 200050 China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/6960.html" title="特种结构材料">特种结构材料;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=capacitance&option=203" rel="nofollow">capacitance;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=dual‐doping&option=203" rel="nofollow">dual‐doping;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=graphene&option=203" rel="nofollow">graphene;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=lithium‐ion batteries&option=203" rel="nofollow">lithium‐ion batteries;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=porous&option=203" rel="nofollow">porous;</a> </p> <div class="translation"> 机译：电容;双掺杂;石墨烯;锂离子电池;多孔; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> 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SECONDARY BATTERIES USING SOLID STATE REACTION AND AN ANODE AND A LITHIUM SECONDARY BATTERY COMPRISING THE ANODE</a> <b>[P]</b> . <span> 外国专利：  KR20160115701A </span> <span> . 2016-10-06</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：利用固相反应制造掺有氮的碳和硅硫化物复合材料作为锂二次电池阳极材料的方法 </span> </p> </li> <li> <div> <b>5. </b><a class="enjiyixqcontent" href="/patent-detail/06130403238378.html">N - Nitrogen doped reduced graphene oxide artificial solid electrolyte interphase and anode for lithium metal battery comprising the same</a> <b>[P]</b> . <span> 外国专利：  KR20190101743A </span> <span> . 2019-09-02</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：N-氮掺杂的还原氧化石墨烯人造固体电解质的界面和包含其的锂金属电池负极 </span> </p> </li> </ul> </div> </div> </div> <div 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