Room‐temperature Synthesis of Amorphous Molybdenum Oxide Nanodots with Tunable Localized Surface Plasmon Resonances

Zhu Chuanhui; Xu Qun; Ji Liang; Ren Yumei; Fang Mingming

摘要

Abstract > Two‐dimensional?(2D) semiconductors have recently emerged as a remarkable class of plasmonic alternative to conventional noble metals. However, tuning of their plasmonic resonances towards different wavelengths in the visible‐light region with physical or chemical methods still remains challenging. In this work, we design a simple room‐temperature chemical reaction route to synthesize amorphous molybdenum oxide (MoO <sub> 3? x </sub> ) nanodots that exhibit strong localized surface plasmon resonances (LSPR) in the visible and near‐infrared region. Moreover, tunable plasmon resonances can be achieved in a wide range with the changing surrounding solvent, and accordingly the photoelectrocatalytic activity can be optimized with the varying LSPR peaks. This work boosts the light–matter interaction at the nanoscale and could enable photodetectors, sensors, and photovoltaic devices in the future. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><abstract xmlns =“http://www.wiley.com/namespaces/wiley”type =“main”xml：lang =“en”> <title type =“main”>抽象</ title> >两个 - 尺寸的尺寸？（2D）半导体最近被成为传统贵金属的非凡等类别的替代品。然而，以物理或化学方法调整朝向可见光区域中的不同波长的等离子体谐振仍然仍然具有挑战性。在这项工作中，我们设计了一种简单的室温化学反应途径，以合成无定形钼（MOO <sub> 3？ X / sub>）纳米型，其表现出强大的局部表面等离子体共振（LSPR）在可见光和近红外区域。此外，可调谐等离子体共振可以在宽范围内实现，随着改变的周围溶剂，因此可以用不同的LSPR峰优化光电催化活性。这项工作提高了纳米级的浅型相互作用，并可在将来能够实现光电探测器，传感器和光伏器件。 </ p> </ abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16161/'>《Chemistry, an Asian journal》</a> <b style="margin: 0 2px;">|</b><span>2017年第23期</span><b style="margin: 0 2px;">|</b><span>共5页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhu Chuanhui&option=202" target="_blank" rel="nofollow">Zhu Chuanhui;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xu Qun&option=202" target="_blank" rel="nofollow">Xu Qun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ji Liang&option=202" target="_blank" rel="nofollow">Ji Liang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ren Yumei&option=202" target="_blank" rel="nofollow">Ren Yumei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Fang Mingming&option=202" target="_blank" rel="nofollow">Fang Mingming;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>College of Materials Science and EngineeringZhengzhou UniversityDaxue Road Zhengzhou 450001 P.R. China;</p> <p>College of Materials Science and EngineeringZhengzhou UniversityDaxue Road Zhengzhou 450001 P.R. China;</p> <p>College of Materials Science and EngineeringZhengzhou UniversityDaxue Road Zhengzhou 450001 P.R. China;</p> <p>College of Materials Science and EngineeringZhengzhou UniversityDaxue Road Zhengzhou 450001 P.R. China;</p> <p>College of Materials Science and EngineeringZhengzhou UniversityDaxue Road Zhengzhou 450001 P.R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/159.html" title="化学">化学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=amorphous&option=203" rel="nofollow">amorphous;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=molybdenum oxides&option=203" rel="nofollow">molybdenum oxides;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanodots&option=203" rel="nofollow">nanodots;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=solar energy utilization&option=203" rel="nofollow">solar energy utilization;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=surface plasmon resonance&option=203" rel="nofollow">surface plasmon resonance;</a> </p> <div class="translation"> 机译：无定形;氧化钼;纳米蛋白;太阳能利用;表面等离子体共振; </div> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022087044.html">Front Cover: Room‐temperature Synthesis of Amorphous Molybdenum Oxide Nanodots with Tunable Localized Surface Plasmon Resonances (Chem. 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target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,樊自拴</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=孙冬柏&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,孙冬柏</a> <span> <a href="/journal-cn-4503/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 北京科技大学学报 </a> </span> <span> . 2005</span><span>,第004期</span> </span> </div> </li> <li> <div> <b>6. </b><a class="enjiyixqcontent" href="/academic-conference-cn_meeting-21617_thesis/02022411293.html">纳米压痕块状非晶合金室温微区形变的研究</a> <b>[C]</b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=杨飞&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 杨飞</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=张微&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,张微</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=杨建林&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">,杨建林</a> <span> <a href="/conference-cn-21617/" target="_blank" rel="nofollow" class="tuijian_authcolor"> . 第四届沈阳科学学术年会 </a> <span> <span> . 2007</span> </span> </div> </li> <li> <div> <b>7. </b><a class="enjiyixqcontent" href="/academic-degree-domestic_mphd_thesis/020314665756.html">室温合成非晶CdO纳米片阵列及其气敏性能研究</a> <b>[A] </b> <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=张叶青&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor"> . 张叶青</a> <span> . 2015</span> </span> </div> </li> </ul> <ul style="display: none;"> <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/patent-detail/061204318713.html">一种金属钼原子掺杂本体氧化钼制备具有LSPR效应的非晶氧化钼纳米片的方法</a> <b>[P]</b> . <span> 中国专利： CN109970103B </span> <span> . 2021.04.02</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120100836749.html">一种金属钼原子掺杂本体氧化钼制备具有LSPR效应的非晶氧化钼纳米片的方法</a> <b>[P]</b> . <span> 中国专利： CN109970103A </span> <span> . 2019-07-05</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130417025852.html">STRUCTURE REPLICATION METHOD, LOCALIZED SURFACE PLASMON RESONANCE SENSOR CHIP MANUFACTURING METHOD INCLUDING THIS REPLICATION METHOD, STRUCTURE, LOCALIZED SURFACE PLASMON RESONANCE SENSOR CHIP, AND LOCALIZED SURFACE PLASMON RESONANCE SENSOR</a> <b>[P]</b> . <span> 外国专利：  WO2014168237A1 </span> <span> . 2014-10-16</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：结构复制方法，局部表面等离子体共振传感器芯片制造方法，包括该复制方法，结构，局部表面等离子体共振传感器芯片和局部表面等离子体共振传感器 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130407455421.html">Localized surface plasmon resonance sensing chip and localized surface plasmon resonance sensing system</a> <b>[P]</b> . <span> 外国专利：  US10001439B2 </span> <span> . 2018-06-19</span> </div> <p 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