An Eco‐Friendly Nitrogen Source for the Preparation of Vanadium Nitride/Nitrogen‐Doped Carbon Nanocomposites for Supercapacitors

Jiang Xin; Lu Wei; Li Yunfeng; Yu Yang; Zhou Xuanbo; Liu Xianchun; Xing Yan

摘要

Abstract > It is highly urgent to find an eco‐friendly nitrogen source for the preparation of metal nitrides as an electrode material for supercapacitors (SCs). Herein, vanadium nitride/N‐doped carbon (VN/NC) nanocomposites were prepared from the nitrogen source of g‐C <sub>3</sub> N <sub>4</sub> by a facile one‐step annealing process. VN NPs, with an average particle size of 7?nm, make an important contribution to the capacitance of the composites. N‐doped carbon (NC), with an advanced sheet‐like structure and high nitrogen content provides a large surface area and effective electrolyte penetration, leading to more exposed VN active sites and a good electrical conductivity. As a supporting substrate, NC nanosheets (NCS) prevent VN NPs from aggregation, thereby a favorable cycling stability of the composite electrode was achieved. In addition, as the (?) 0.04‐VN/NCS2//NiCo <sub>2</sub> S <sub>4</sub> (+) asymmetric device is assembled, favorable specific capacitance, high energy, and power density can also be obtained. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 找到一种用于制备金属氮化物作为超级电容器（SCS）的电极材料的生态型氮源是高迫切的。这里，由G-C的氮来源制备氮化钒/ n掺杂的碳（VN / NC）纳米复合材料 <sub> 3 </ sub> N. <sub> 4 </ sub> 通过便利的一步退火过程。 VN NPS，平均粒径为7Ω·Nm，对复合材料的电容作出了重要贡献。具有先进的片状结构和高氮含量的N-掺杂的碳（NC）提供了大的表面积和有效电解质渗透，导致更暴露的VN活性位点和良好的导电性。作为支撑衬底，NC纳米晶片（NCS）可防止VN NPS聚集，从而实现了复合电极的良好循环稳定性。另外，作为（？）0.04-Vn / ncs2 // nico <sub> 2 </ sub> S. <sub> 4 </ sub> （+）不对称装置被组装，有利的特定电容，高能量和功率密度也可以获得。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16042/'>《ChemElectroChem》</a> <b style="margin: 0 2px;">|</b><span>2019年第13期</span><b style="margin: 0 2px;">|</b><span>共9页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jiang Xin&option=202" target="_blank" rel="nofollow">Jiang Xin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lu Wei&option=202" target="_blank" rel="nofollow">Lu Wei;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Yunfeng&option=202" target="_blank" rel="nofollow">Li Yunfeng;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Yu Yang&option=202" target="_blank" rel="nofollow">Yu Yang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhou Xuanbo&option=202" target="_blank" rel="nofollow">Zhou Xuanbo;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Liu Xianchun&option=202" target="_blank" rel="nofollow">Liu Xianchun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Xing Yan&option=202" target="_blank" rel="nofollow">Xing Yan;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Chemistry Northeast Normal UniversityJilin Provincial Key Laboratory of Advanced Energy MaterialsChangchun 130024 P. R. China;</p> <p>Department of Chemistry Northeast Normal UniversityJilin Provincial Key Laboratory of Advanced Energy MaterialsChangchun 130024 P. R. China;</p> <p>College of Environmental and Chemical EngineeringXi'an Polytechnic UniversityXi'an 710000 P. R. China;</p> <p>Department of Chemistry Northeast Normal UniversityJilin Provincial Key Laboratory of Advanced Energy MaterialsChangchun 130024 P. R. China;</p> <p>Department of Chemistry Northeast Normal UniversityJilin Provincial Key Laboratory of Advanced Energy MaterialsChangchun 130024 P. R. China;</p> <p>Department of Chemistry Northeast Normal UniversityJilin Provincial Key Laboratory of Advanced Energy MaterialsChangchun 130024 P. R. China;</p> <p>Department of Chemistry Northeast Normal UniversityJilin Provincial Key Laboratory of Advanced Energy MaterialsChangchun 130024 P. R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=vanadium nitride&option=203" rel="nofollow">vanadium nitride;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=N-doped carbon&option=203" rel="nofollow">N-doped carbon;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=g-C3N4&option=203" rel="nofollow">g-C3N4;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=nanocomposite&option=203" rel="nofollow">nanocomposite;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=supercapacitors&option=203" rel="nofollow">supercapacitors;</a> </p> <div class="translation"> 机译：氮化钒;n掺杂的碳;g-c3n4;纳米复合材料;超级电容器; </div> </li> </ul> </div> </div> <div class="literature cardcommon" id="literaturereference" style="display:none"> <div class="similarity "> <h3 class="all_title" id="enpatent111">引文网络</h3> <div class="referencetab clearfix"> <ul id="referencedaohang"> <li dataid="referenceul">参考文献</li> <li dataid="citationul">引证文献</li> <li dataid="commonreferenceul">共引文献</li> <li dataid="commoncitationul">同被引文献</li> <li dataid="tworeferenceul">二级参考文献</li> <li dataid="twocitationul">二级引证文献</li> </ul> </div> <div class="reference_details" id="referenceList"> <ul id="referenceul"></ul> <ul id="citationul"></ul> <ul id="commonreferenceul"></ul> <ul id="commoncitationul"></ul> <ul id="tworeferenceul"></ul> <ul id="twocitationul"></ul> </div> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/academic-journal-cn_transactions-nonferrous-metals-society-china_thesis/0201289457064.html">用于氧还原反应的氮掺杂空心多孔碳球封装的过渡金属氮化物的制备和性能</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=李彦娟&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">李彦娟,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=王敏&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">王敏,</a> 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