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Synthesis of a Novel Petal‐Shaped Biomass‐Derived Carbon Material with Controlled Pore Structure and Nitrogen Content for Use in Supercapacitors

机译：合成具有控制孔结构的新型花瓣状生物质衍生的碳材料和用于超级电容器的氮含量

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摘要

Abstract > Controllably adjusting the porosity and the heteroatom content has become extremely attractive for increasing the energy storage capacity of carbon materials. In this work, petal‐shaped N‐doping carbon materials with super‐high specific surface area (2752?m 2 ?g ?1 ) and enriched micropores (90.1?%) have been synthesized by using renewable spikes of terminalia catappa as raw materials via a facile and feasible method. The results confirmed that the prepared N‐doping carbon material exhibits outstanding electrochemical performances. The specific capacitance reaches up to 503?F?g ?1 at 0.5?A?g ?1 and 306?F?g ?1 at 50?A?g ?1 ; cycling stability maintains 100.2?% after 10000 cycles. The fabricated symmetric supercapacitor shows an attractive energy density of 30.5?W?h?Kg ?1 at a power density of 492.4?W?Kg ?1 in 1?M Na <sub>2</sub> SO <sub>4</sub> electrolyte. Moreover, this study opens up a new way to enhance the micropore proportion and N content of carbon materials and displays the unique petal‐shaped nano‐flakes morphology that can maximally expose the surface of carbon materials. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 可控地调节孔隙率和杂原子含量对于增加碳材料的能量储存能力而变得极其吸引力。在这项工作中，花瓣形的n掺杂碳材料，具有超高比表面积（2752？m 2 </ sup> ？G ？1 </ sup> ）通过使用容易和可行的方法使用可再生峰值作为原料来合成富集的微孔（90.1〜Δ％）。结果证实，制备的N-掺杂碳材料表现出出色的电化学性能。具体电容达到503？f？g ？1 </ sup> 0.5？a？g ？1 </ sup> 和306？f？g ？1 </ sup> 50？a？g ？1 </ sup> ;循环稳定性在10000次循环后保持100.2倍。制造的对称超级电容器显示出30.5Ω的有吸引力的能量密度为30.5？H？kg ？1 </ sup> 功率密度为492.4？w？kg ？1 </ sup> 在1？m na <sub> 2 </ sub> 所以 <sub> 4 </ sub> 电解质。此外，该研究开辟了一种新的方式来增强碳材料的微孔比例和N含量，并显示出可以最大地暴露碳材料表面的独特花瓣状纳米片形态。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16042/'>《ChemElectroChem》</a> <b style="margin: 0 2px;">|</b><span>2019年第23期</span><b style="margin: 0 2px;">|</b><span>共10页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Luming&option=202" target="_blank" rel="nofollow">Zhang Luming;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Zhang Xiaohua&option=202" target="_blank" rel="nofollow">Zhang Xiaohua;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Tian Xin&option=202" target="_blank" rel="nofollow">Tian Xin;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Wang Qun&option=202" target="_blank" rel="nofollow">Wang Qun;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Li Hengxiang&option=202" target="_blank" rel="nofollow">Li Hengxiang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jin Lie&option=202" target="_blank" rel="nofollow">Jin Lie;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cao Qing&option=202" target="_blank" rel="nofollow">Cao Qing;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Institute of Chemistry and Chemical EngineeringTaiyuan University of TechnologyShanxi 030024 P.R. China;</p> <p>Institute of Chemistry and Chemical EngineeringTaiyuan University of TechnologyShanxi 030024 P.R. China;</p> <p>Institute of Chemistry and Chemical EngineeringTaiyuan University of TechnologyShanxi 030024 P.R. China;</p> <p>Institute of Chemistry and Chemical EngineeringTaiyuan University of TechnologyShanxi 030024 P.R. China;</p> <p>Institute of Chemistry and Chemical EngineeringTaiyuan University of TechnologyShanxi 030024 P.R. China;</p> <p>Institute of Chemistry and Chemical EngineeringTaiyuan University of TechnologyShanxi 030024 P.R. China;</p> <p>Institute of Chemistry and Chemical EngineeringTaiyuan University of TechnologyShanxi 030024 P.R. China;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=carbon flakes&option=203" rel="nofollow">carbon flakes;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=biomass-derived carbon&option=203" rel="nofollow">biomass-derived carbon;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=pore adjustment&option=203" rel="nofollow">pore adjustment;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=N-doping&option=203" rel="nofollow">N-doping;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=supercapacitor&option=203" rel="nofollow">supercapacitor;</a> </p> <div class="translation"> 机译：碳薄片;生物量衍生的碳;孔隙调节;n-掺杂;超级电容器; </div> </li> <li> <span class="lefttit">入库时间</span> <span>2022-08-19 23:30:10</span> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022060460.html">Synthesis of a Novel Petal‐Shaped Biomass‐Derived Carbon 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