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Tapping Renewables: A New Dawn for Organic Electrosynthesis in Aqueous Reaction Media

机译：攻丝可再生能源：在水性反应介质中有机电气合成的新曙光

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Abstract >The birthplace of organic electrochemistry was an aqueous solution, with a biogenic, renewable compound being the reactant of the first organic electrosynthesis. Now, 170?years later, the relevance of electrosynthesis is rising again and, hence, the original work comes to the fore. Water is considered a green solvent, biogenic compounds increasingly replace fossil compounds as a feedstock for the chemical industry, and electrosynthesis bridges energy and chemistry sector. In this Minireview, we advocate the use of water as the solvent for electrochemical conversion of biogenic organic compounds. We show that, although the use of water may put certain constraints on organic electrosynthesis, using aqueous reaction media opens interesting perspectives. As illustrated on selected examples, synergies can be created for the conversion of oxygenates, for hydrogenation and hydrodeoxygenation reactions, product separation and in coupling electrochemical and biochemical processes. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> >有机电化学的出生地是一种水溶液，具有生物，可再生化合物，是第一有机电气合成的反应物。现在，170年后，电气合成的相关性再次升起，因此原始工作达到前。水被认为是一种绿色溶剂，生物化合物越来越替代化石化合物作为化学工业原料，电动交织桥接能量和化学部门。在这次MILEVIEW中，我们倡导使用水作为生物原性有机化合物的电化学转化的溶剂。我们表明，尽管使用水可以对有机电气合成的某些约束，但使用水性反应培养基开启有趣的观点。如所选择的实施例所示，可以为含氧化合物的转化产生协同作用，用于氢化和加氢脱氧反应，产物分离和偶联电化学和生物化学过程。</ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16042/'>《ChemElectroChem》</a> <b style="margin: 0 2px;">|</b><span>2019年第16期</span><b style="margin: 0 2px;">|</b><span>共8页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Harnisch Falk&option=202" target="_blank" rel="nofollow">Harnisch Falk;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Schr?der Uwe&option=202" target="_blank" rel="nofollow">Schr?der Uwe;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>Department of Environmental MicrobiologyHelmholtz-Centre for Environmental Research – UFZPermoserstrasse 15 04318 Leipzig Germany;</p> <p>Institute of Environmental and Sustainable ChemistryTechnische Universit?t BraunschweigHagenring 30 38106 Braunschweig Germany;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrosynthesis&option=203" rel="nofollow">electrosynthesis;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=renewables&option=203" rel="nofollow">renewables;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrobiorefinieries&option=203" rel="nofollow">electrobiorefinieries;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=electrochemical oxidation&option=203" rel="nofollow">electrochemical oxidation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=hydrogenation&option=203" rel="nofollow">hydrogenation;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=water&option=203" rel="nofollow">water;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=green chemistry&option=203" rel="nofollow">green chemistry;</a> </p> <div class="translation"> 机译：电动合成;可再生能源;电化无晶体;电化学氧化;氢化;水;绿色化学; </div> </li> <li> <span class="lefttit">入库时间</span> <span>2022-08-19 23:30:10</span> </li> </ul> </div> </div> <div class="literature cardcommon"> <div class="similarity "> <h3 class="all_title" id="enpatent66">相似文献</h3> <div class="similaritytab clearfix"> <ul> <li class="active" >外文文献</li> <li >中文文献</li> <li >专利</li> </ul> </div> <div class="similarity_details"> <ul > <li> <div> <b>1. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704022060440.html">Tapping Renewables: A New Dawn for Organic Electrosynthesis in Aqueous Reaction Media</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Harnisch Falk&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Harnisch Falk,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Schr?der Uwe&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Schr?der Uwe </a> <a href="/journal-foreign-16042/" target="_blank" rel="nofollow" class="tuijian_authcolor">ChemElectroChem .</a> <span>2019</span><span>,第16期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：攻丝可再生能源：在水性反应介质中有机电气合成的新曙光</span> </p> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/journal-foreign-detail/0704013600381.html">Electrosynthesis of hydrogen peroxide in acidic solutions by mediated oxygen reduction in a three-phase (aqueous/organic/gaseous) system - Part I: Emulsion structure, electrode kinetics and batch electrolysis</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Gyenge EL.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Gyenge EL.,</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Oloman W.&option=202" target="_blank" rel="nofollow" class="tuijian_auth tuijian_authcolor">Oloman W. </a> <a href="/journal-foreign-33555/" target="_blank" rel="nofollow" class="tuijian_authcolor">Journal of Applied Electrochemistry .</a> <span>2003</span><span>,第8期</span> </span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：三相（水/有机/气态）系统中介导的氧还原在酸性溶液中电合成过氧化氢-第一部分：乳液结构，电极动力学和间歇电解</span> </p> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/academic-journal-foreign_journal-applied-electrochemistry_thesis/0204110476833.html">Electrosynthesis of hydrogen peroxide in acidic solutions by mediated oxygen reduction in a three-phase (aqueous/organic/gaseous) system Part I: Emulsion structure, electrode kinetics and batch electrolysis</a> <b>[J]</b> . <span> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=E.L. 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href="/patent-detail/061203658422.html">使用胶体沉淀碳酸钙吸附水性介质中的有机物质和/或减少水性介质中有机物质的量</a> <b>[P]</b> . <span> 中国专利： CN106232527B </span> <span> . 2020.03.06</span> </div> </li> <li> <div> <b>2. </b><a class="enjiyixqcontent" href="/patent-detail/06120108722960.html">使用胶体沉淀碳酸钙吸附水性介质中的有机物质和/或减少水性介质中有机物质的量</a> <b>[P]</b> . <span> 中国专利： CN106232527A </span> <span> . 2016-12-14</span> </div> </li> <li> <div> <b>3. </b><a class="enjiyixqcontent" href="/patent-detail/06130495441600.html">Effecting organic reactions in aqueous media at high temperatures</a> <b>[P]</b> . <span> 外国专利：  US1868140A </span> <span> . 1932-07-19</span> </div> <p class="zwjiyix translation" style="max-width: initial;height: auto;word-break: break-all;white-space: initial;text-overflow: initial;overflow: initial;"> <span>机译：在高温下在水性介质中影响有机反应 </span> </p> </li> <li> <div> <b>4. </b><a class="enjiyixqcontent" href="/patent-detail/06130461784678.html">Reactor for the use of immobilized enzymes in a continuous flow reaction (FIA) 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