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Cu ₂2 O Photocathode with Faster Charge Transfer by Fully Reacted Cu Seed Layer to Enhance Performance of Hydrogen Evolution in Solar Water Splitting Applications

机译：铜 _{2 2 o通过完全反应的Cu种子层具有更快的电荷转移的光电处理，以提高太阳能水分裂应用中氢气进化的性能}

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Abstract > In this work, we study the effect of Cu <sub>2</sub> O film obtained from a fully reacted Cu seed layer as a photoelectrode in photoelectrochemical cells. The full reaction of the Cu layer shows an enhanced photocurrent density and improved efficiency in hydrogen evolution. The photocurrent density of textured Cu <sub>2</sub> O (0.58?mA?cm ?2 at 0?V vs. RHE), without an unreacted Cu layer is two times higher than films containing an unreacted Cu layer (0.29?mA?cm ?2 at 0?V vs. RHE), under AM 1.5 illumination (100?mW?cm ?2 ). The thickness of the unreacted Cu layer influences significantly the charge transfer process at the interface between the Cu <sub>2</sub> O and electrolyte. The enhanced photoelectrochemical performance of textured Cu <sub>2</sub> O is attributed to the reduced charge recombination resulting from a longer carrier lifetime in the Cu <sub>2</sub> O layer. Experimentally we confirmed that the unreacted Cu layer inhibits the photoelectrochemical performance of Cu <sub>2</sub> O‐based photocathodes. The elimination of the unreacted Cu layer leads to higher photocurrent density. </abstract> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> <div class="translation abstracttxt"> <span class="zhankaihshouqi fivelineshidden" id="abstract"> <span>机译：</span><Abstract Type =“Main”XML：Lang =“en”> <标题类型=“main”>抽象</ title> > 在这项工作中，我们研究了Cu的影响 <sub> 2 </ sub> o从完全反应的Cu种子层获得的膜作为光电子细胞中的光电极。 Cu层的完全反应显示出增强的光电流密度和氢气进化的提高效率。纹理Cu的光电流密度 <sub> 2 </ sub> o（0.58？ma？cm ？2 </ sup> 在0？v与Rhe），没有未反应的Cu层的比含有未反应的Cu层的薄膜高出两倍（0.29≤CA ？2 </ sup> 在0？v与rhe）下，下午1.5照明（100？mw？cm ？2 </ sup> ）。未反应的Cu层的厚度显着影响Cu之间接口处的电荷转移过程 <sub> 2 </ sub> o和电解质。增强纹理Cu的光电化学性能 <sub> 2 </ sub> o归因于由Cu中的较长载体寿命产生的减少的电荷重组 <sub> 2 </ sub> o层。实验我们证实未反应的Cu层抑制了Cu的光电化学性能 <sub> 2 </ sub> 基于O基光电阴极。消除未反应的Cu层导致更高的光电流密度。 </ p> </摘要> </span> <span class="z_kbtn z_kbtnclass hoverxs" style="display: none;">展开▼</span> </div> </div> <div class="record"> <h2 class="all_title" id="enpatent33" >著录项</h2> <ul> <li> <span class="lefttit">来源</span> <div style="width: 86%;vertical-align: text-top;display: inline-block;"> <a href='/journal-foreign-16041/'>《ChemCatChem》</a> <b style="margin: 0 2px;">|</b><span>2019年第17期</span><b style="margin: 0 2px;">|</b><span>共6页</span> </div> </li> <li> <div class="author"> <span class="lefttit">作者</span> <p id="fAuthorthree" class="threelineshidden zhankaihshouqi"> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Jung Kichang&option=202" target="_blank" rel="nofollow">Jung Kichang;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Lim Taehoon&option=202" target="_blank" rel="nofollow">Lim Taehoon;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Bae Hyojung&option=202" target="_blank" rel="nofollow">Bae Hyojung;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Ha Jun‐Seok&option=202" target="_blank" rel="nofollow">Ha Jun‐Seok;</a> <a href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Martinez‐Morales Alfredo A.&option=202" target="_blank" rel="nofollow">Martinez‐Morales Alfredo A.;</a> </p> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zkzz" style="display: none;">展开▼</span> </div> </li> <li> <div style="display: flex;"> <span class="lefttit">作者单位</span> <div style="position: relative;margin-left: 3px;max-width: 639px;"> <div class="threelineshidden zhankaihshouqi" id="fOrgthree"> <p>College of Engineering- Center for Environmental Research &</p> <p>TechnologyUniversity of California Riverside1084 Columbia Ave. Riverside CA 92507 USA;</p> <p>College of Engineering- Center for Environmental Research &</p> <p>TechnologyUniversity of California Riverside1084 Columbia Ave. Riverside CA 92507 USA;</p> <p>Optoelectronics Convergence Research CenterChonnam National University77 Yongbong-ro Buk-gu Gwangju 61186 Republic of Korea;</p> <p>Optoelectronics Convergence Research CenterChonnam National University77 Yongbong-ro Buk-gu Gwangju 61186 Republic of Korea;</p> <p>College of Engineering- Center for Environmental Research &</p> <p>TechnologyUniversity of California Riverside1084 Columbia Ave. Riverside CA 92507 USA;</p> </div> <span class="z_kbtnclass z_kbtnclassall hoverxs" id="zhdw" style="display: none;">展开▼</span> </div> </div> </li> <li > <span class="lefttit">收录信息</span> <span style="width: 86%;vertical-align: text-top;display: inline-block;"></span> </li> <li> <span class="lefttit">原文格式</span> <span>PDF</span> </li> <li> <span class="lefttit">正文语种</span> <span>eng</span> </li> <li> <span class="lefttit">中图分类</span> <span><a href="https://www.zhangqiaokeyan.com/clc/1186.html" title="物理化学（理论化学）、化学物理学">物理化学（理论化学）、化学物理学;</a></span> </li> <li class="antistop"> <span class="lefttit">关键词</span> <p style="width: 86%;vertical-align: text-top;"> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Hydrogen evolution&option=203" rel="nofollow">Hydrogen evolution;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Photoelectrocatalyst&option=203" rel="nofollow">Photoelectrocatalyst;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=Cu 2 O&option=203" rel="nofollow">Cu 2 O;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=metal-oxide catalyst&option=203" rel="nofollow">metal-oxide catalyst;</a> <a style="color: #3E7FEB;" href="/search.html?doctypes=4_5_6_1-0_4-0_1_2_3_7_9&sertext=photocatalyst&option=203" rel="nofollow">photocatalyst;</a> </p> <div class="translation"> 机译：氢气进化;光电催化剂;Cu 2 O;金属氧化物催化剂;光催化剂; 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Cu 22 O Photocathode with Faster Charge Transfer by Fully Reacted Cu Seed Layer to Enhance Performance of Hydrogen Evolution in Solar Water Splitting Applications

摘要

Cu ₂2 O Photocathode with Faster Charge Transfer by Fully Reacted Cu Seed Layer to Enhance Performance of Hydrogen Evolution in Solar Water Splitting Applications