Modelling intragranular fission gas release in irradiation of sintered LWR UO2 fuel

摘要

A model for the release of stable fission gases by diffusion from sintered LWR UO2 fuel grains is presented. The model takes into account intragranular gas bubble behaviour as a function of grain radius. The bubbles are assumed to be immobile and the gas migrates to grain boundaries by diffusion of single gas atoms. The intragranular bubble population in the model at low burn-ups or temperatures consists of numerous small bubbles. The presence of the bubbles attenuates the effective gas atom diffusion coefficient. Rapid coarsening of the bubble population in increased burn-up at elevated temperatures weakens significantly the attenuation of the effective diffusion coefficient. The solution method introduced in earlier papers, locally accurate method, is enhanced to allow accurate calculation of the intragranular gas behaviour in time varying conditions without excessive computing time. Qualitatively the detailed model can predict the gas retention in the grain better than a more simple model. (C) 2002 Elsevier Science B.V. All rights reserved. [References: 68]