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Fluctuations of jamming coverage upon random sequential adsorption on homogeneous and heterogeneous media - art. no. 041106

机译:在均相和非均相介质上随机顺序吸附后的干扰覆盖范围波动-art。没有。 041106

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摘要

The fluctuations of the jamming coverage upon random sequential adsorption (RSA) are studied using both analytical and numerical techniques. Our main result shows that these fluctuations (characterized by sigma(thetaJ)) decay with the lattice size according to the power law sigma(thetaJ)proportional toL(-1u). The exponent nu depends on the dimensionality D of the substrate and the fractal dimension of the set where the RSA process actually takes place (d(f)) according to nu=2/(2D-d(f)). This theoretical result is confirmed by means of extensive numerical simulations applied to the RSA of dimers on homogeneous and stochastic fractal substrates. Furthermore, our predictions are in excellent agreement with different previous numerical results. It is also shown that, studying correlated stochastic processes, one can define various fluctuating quantities designed to capture either the underlying physics of individual processes or that of the whole system. So, subtle differences in the definitions may lead to dramatically different physical interpretations of the results. Here, this statement is demonstrated for the case of RSA of dimers on binary alloys. [References: 25]
机译:使用分析和数值技术研究了随机顺序吸附(RSA)时干扰覆盖率的波动。我们的主要结果表明,这些波动(以sigma(thetaJ)为特征)根据幂定律sigma(thetaJ)与L(-1 / nu)成正比,随晶格大小而衰减。指数nu取决于基板的尺寸D和根据nu = 2 /(2D-d(f))实际进行RSA处理的设备的分形尺寸(d(f))。通过对均质和随机分形底物上二聚体的RSA进行广泛的数值模拟,证实了这一理论结果。此外,我们的预测与以前的不同数值结果非常吻合。还表明,研究相关的随机过程,可以定义各种波动量,这些波动量旨在捕获单个过程或整个系统的基础物理。因此,定义中的细微差异可能会导致结果的物理解释发生显着不同。在此,针对二元合金上二聚体的RSA情况证明了这一说法。 [参考:25]

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