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首页> 外文期刊>Physical Review, A. Atomic, molecular, and optical physics >Strong-field ionization with two-color circularly polarized laser fields
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Strong-field ionization with two-color circularly polarized laser fields

机译:两色圆偏振激光场的强场电离

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Strong-field ionization provides fundamental insight into light-matter interactions, encoding the structure of atoms and molecules on the subangstrom and subfemtosecond scales. In this Rapid Communication, we explore an important regime: strong-field ionization by two-color circularly polarized laser fields. In contrast to past work using linearly polarized drivers, we probe electron trajectories that are driven in a two-dimensional plane, thus separating the tunneling angle from the rescattering angle. This allows us to make several findings. First, we observe a single-lobed electron distribution for co-rotating fields, and a three-lobed distribution for counter-rotating fields, providing experimental validation of the theoretical model explaining the generation of circularly polarized high harmonic light. Second, we discover that there is significant electron-ion rescattering using counter-rotating fields, but not with co-rotating fields. Finally, we show that the rescattered electrons are well separated from the directly ionized electrons, in striking contrast to similar low-energy structures seen with linearly polarized fields. These findings help overcome the long-standing problem of how to decouple the tunneling and rescattering steps in strong-field ionization, which will enable new dynamic probes of atomic and molecular structure.
机译:强场电离可提供对光与物质相互作用的基本了解,可在亚埃和亚飞秒范围内编码原子和分子的结构。在本快速通信中,我们探索了一个重要的机制:通过双色圆偏振激光场进行的强场电离。与过去使用线性极化驱动器进行的工作相反,我们探测在二维平面中驱动的电子轨迹,从而将隧穿角与散射角分开。这使我们可以得出一些发现。首先,我们观察到同向旋转场的单瓣电子分布和反向旋转场的三瓣电子分布,为解释圆偏振高谐波光的产生的理论模型提供了实验验证。其次,我们发现使用反向旋转场会产生明显的电子离子散射,而使用反向旋转场则不会。最后,我们证明了散射的电子与直接电离的电子之间有很好的隔离,这与线性极化场中看到的类似低能结构形成了鲜明的对比。这些发现有助于克服长期存在的问题,即在强场电离中如何解耦隧穿和散射步骤,这将使原子和分子结构的新动态探针成为可能。

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