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Intriguing electron correlation effects in the photoionization of metallic quantum-dot nanorings

机译:金属量子点纳米环光电离中有趣的电子相关效应

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We report detailed results on ionization in metallic quantum-dot (QD) nanorings described by the extended Hubbard model at half filling obtained by exact numerical diagonalization. In spite of very strong electron correlations, the ionization spectra are astonishingly scarce. We attribute this scarcity to a hidden quasi-symmetry, generalizing thereby similar results on optical absorption recently reported [Phys. Rev. B 75, 125323 (2007); 77, 165339 (2008)]. Numerical results indicate that this hidden quasi-symmetry of the extended Hubbard model does not evolve into a true (hidden) symmetry but remains a quasi-symmetry in the case of the restricted Hubbard model as well. Based on the observation on the number of significant ionization signals per each spatial symmetry, we claim the existence of a one-to-one map between the relevant ionization signals of the correlated half-filled nanorings and the one-hole and two-hole-one_particle processes possible in the noninteracting case. Similar to the case of optical absorption, numerous avoided crossings (anticrossings) are present in the ionization spectra, which often involve more than two states. The present results demonstrate that ionization could be a useful tool to study electron correlations in metallic QD-nanoarrays, providing information that is complementary to optical absorption.
机译:我们报告了由扩展的Hubbard模型描述的金属量子点(QD)纳米环中电离的详细结果,该过程是通过精确数值对角化获得的半填充。尽管电子相关性非常强,但电离光谱却非常稀少。我们将这种稀缺性归因于隐藏的准对称性,从而概括了最近报道的关于光吸收的相似结果。 B 75,125323(2007); 77,165339(2008)]。数值结果表明,扩展的Hubbard模型的这种隐藏的拟对称性不会演变为真实的(隐藏的)对称性,但在受限的Hubbard模型的情况下仍保持为准对称性。基于对每个空间对称性的重要电离信号的数量的观察,我们主张在相关的半填充纳米环的相关电离信号与一个孔和两个孔之间存在一对一的映射在非交互情况下,one_particle处理是可能的。类似于光吸收的情况,电离光谱中存在许多避免的交叉(反交叉),通常涉及两个以上的状态。目前的结果表明,电离可以成为研究金属QD纳米阵列中电子相关性的有用工具,提供与光吸收互补的信息。

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