An integrated campaign for investigation of winter-time continental haze over Indo-Gangetic Basin and its radiative effects

摘要

An outflow of continental haze occurs from Indo-Gangetic Basin (IGB) in the North to Bay of Bengal (BoB) in the South. An integrated campaign was organized to investigate this continental haze during December 2013-February 2014 at source and remote regions within IGB to quantify its radiative effects. Measurements were carried out at three locations in eastern India; 1) Kalas Island, Sundarban (21.68°N, 88.57°E) - an isolated island along the north-east coast of BoB, 2) Kolkata (22.57°N, 88.42°E) - an urban metropolis and 3) Siliguri (26.70°N, 88.35°E) - an urban region at the foothills of eastern Himalayas. Ground-based AOD (at 0.5 μm) is observed to be maximum (1.25 ± 0.18) over Kolkata followed by Siliguri (0.60 ± 0.17) and minimum over Sundarban (0.53 ± 0.18). Black carbon concentration is found to be maximum at Kolkata (21.6 ± 6.6 μg·m~(-3)) with almost equal concentrations at Siliguri (12.6 ± 5.2 μg·m~(-3)) and Sundarban (12.3 ± 3.0 μg·m~(-3)). Combination of MODIS-AOD and back-trajectories analysis shows an outflow of winter-time continental haze originating from central IGB and venting out through Sundarban towards BoB. This continental haze with high extinction coefficient is identified up to central BoB using CALIPSO observations and is found to contribute -75% to marine AOD over central BoB. This haze produces significantly high aerosol radiative forcing within the atmosphere over Kolkata (75.4 Wm~(-2)) as well as over Siliguri and Sundarban (40 Wm~(-2)) indicating large forcing over entire IGB, from foothills of the Himalayas to coastal region. This winter-time continental haze also causes about similar radiative heating (1.5 K·day~(-1)) from Siliguri to Sundarban which is enhanced over Kolkata (3 K·day~(-1)) due to large emission of local urban aerosols. This high aerosol heating over entire IGB and coastal region of BoB can have considerable impact on the monsoonal circulation and more importantly, such haze transported over to BoB can significantly affect the marine hydrological cycle.