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Quantifying and controlling the magnetic dipole contribution to 1.5-μm light emission in erbium-doped yttrium oxide

机译:量化和控制磁di对掺氧化钇中1.5μm发光的贡献

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摘要

We experimentally quantify the contribution of magnetic dipole (MD) transitions to the near-infrared light emission from trivalent erbium-doped yttrium oxide (Er~(3+):Y_2O_3). Using energy-momentum spectroscopy, we demonstrate that the ~4I_(13/2) →4I_(15/2) emission near 1.5 μm originates from nearly equal contributions of electric dipole (ED) and MD transitions that exhibit distinct emission spectra. We then show how these distinct spectra, together with the differing local density of optical states for ED and MD transitions, can be leveraged to control Er~(3+) emission in structured environments. We demonstrate that far-field emission spectra can be tuned to resemble almost pure emission from either ED or MD transitions and show that the observed spectral modifications can be accurately predicted from the measured ED and MD intrinsic emission rates.
机译:我们实验上量化了磁偶极(MD)跃迁对三价掺-氧化钇(Er〜​​(3 +):Y_2O_3)对近红外光发射的贡献。使用能量动量光谱,我们证明了在1.5μm附近的〜4I_(13/2)→4I_(15/2)发射源于表现出不同发射光谱的电偶极(ED)和MD跃迁几乎相等的贡献。然后,我们展示了如何利用这些不同的光谱以及ED和MD跃迁的不同光学态局部密度,来控制结构化环境中的Er〜(3+)发射。我们证明,远场发射光谱可以调整为类似于ED或MD跃迁的几乎纯净的发射,并且表明可以从测得的ED和MD固有发射率准确预测观察到的光谱变化。

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