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Enhanced photocatalytic degradation of methyl orange in TiO_2(B)@anatase heterostructure nanocomposites prepared by a facile hydrothermal method

机译:简便水热法制备的TiO_2(B)@锐钛矿异结构纳米复合材料中甲基橙的光催化降解作用

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摘要

In this work, one-dimensional TiO_2(B)@anatase heterostructure nanocomposites were synthesized via a facile hydrothermal process in ethanol/water solution with the aid of polyvinylpyrrolidone. TiO_2(B) nanobelts were uniformly coated with an anatase nanocrystals shell. The shell thickness can be tuned from 10 nm to 30 nm. The energy bandgap at the heterostructure interface favors the transferring of the photo-induced holes in anatase to TiO_2(B) nanobelts, thus the charge recombination can be effectively suppressed. The nanocomposites showed superior photocatalytic degradation of methyl orange due to the enhanced charge separation efficiency.
机译:在这项工作中,借助聚乙烯吡咯烷酮在乙醇/水溶液中通过简便的水热过程合成了一维TiO_2(B)@锐钛矿异质结构纳米复合材料。 TiO_2(B)纳米带均匀地涂覆有锐钛矿型纳米晶体壳。外壳厚度可以从10 nm调整到30 nm。异质结构界面处的能带隙有利于锐钛矿中光致空穴向TiO_2(B)纳米带的转移,因此可以有效地抑制电荷复合。由于增强的电荷分离效率,纳米复合材料表现出优异的甲基橙光催化降解。

著录项

  • 来源
    《Materials Letters》 |2013年第1期|173-176|共4页
  • 作者单位

    State Key Laboratory of Silicon Materials, Department of Materials Science and Engineering, Zhejiang University, Hangzhou 310027, China;

    State Key Laboratory of Silicon Materials, Department of Materials Science and Engineering, Zhejiang University, Hangzhou 310027, China;

    Department of Physics, Zhejiang University, Hangzhou 310027, China;

    State Key Laboratory of Silicon Materials, Department of Materials Science and Engineering, Zhejiang University, Hangzhou 310027, China;

    State Key Laboratory of Silicon Materials, Department of Materials Science and Engineering, Zhejiang University, Hangzhou 310027, China;

    State Key Laboratory of Silicon Materials, Department of Materials Science and Engineering, Zhejiang University, Hangzhou 310027, China;

    State Key Laboratory of Silicon Materials, Department of Materials Science and Engineering, Zhejiang University, Hangzhou 310027, China;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    Hydrothermal; TiO_2(B); Anatase; Photocatalysis; Semiconductors; Nanocomposites;

    机译:水热TiO_2(B);锐钛矿;光催化;半导体;纳米复合材料;

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