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Novel BeZnO Based Self-Powered Dual-Color UV Photodetector Realized via a One-Step Fabrication Method

机译:通过一步制造方法实现的新型基于BeZnO的自供电双色UV光电探测器

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In this work, we fabricated a novel BeZnO based dual-color UV photodetector through a one-step electron beam evaporation of asymmetric Ti/Au pair. A dual-phase BeZnO alloy film with dual bandgap of similar to 3.5 eV (similar to 355 nm) and similar to 4.6 eV(similar to 270 nm) was artfully utilized as active layer to realize dual-color response. This photodetector shows a noticeable photovoltaic characteristic and can be utilized as an excellent self-powered device. The device exhibits two cut-off response wavelengths at similar to 275 nm and similar to 360 nm under zero bias, which are corresponding to UVA and UVC region, respectively. According to the dynamic response spectra under UV radiation, the device presents excellent stability and reproducibility without external power supply. In addition, the device has an ultrafast response speed, with a rise time of similar to 35 mu s and a decay time of similar to 880 mu s. Finally, a physical model based on energy band theory is proposed to demonstrate that the self-powered behavior is attributed to the asymmetric Schottky barrier heights caused by the hole-trapping process occurred in electrode/BeZnO interface. To the best of our knowledge, this is the first report on BeZnO based self-powered UV photodetector. Our findings demonstrate a novel and facile route to realize high performance self-powered UV photodetectors for multipurposes.
机译:在这项工作中,我们通过不对称Ti / Au对的一步电子束蒸发制备了一种新颖的基于BeZnO的双色UV光电探测器。巧妙地采用双带隙近似于3.5 eV(近似于355 nm)和近似4.6 eV(近似于270 nm)的双相BeZnO合金膜作为有源层,以实现双色响应。该光电探测器具有明显的光伏特性,可以用作出色的自供电设备。该器件在零偏置下显示出两个截止响应波长,分别类似于275 nm和360 nm,分别对应于UVA和UVC区域。根据紫外线辐射下的动态响应光谱,该器件无需外部电源即可提供出色的稳定性和可重复性。此外,该设备具有超快的响应速度,上升时间类似于35毫秒,衰减时间类似于880毫秒。最后,提出了一种基于能带理论的物理模型,证明了自供电行为归因于电极/ BeZnO界面中发生的空穴俘获过程引起的不对称肖特基势垒高度。据我们所知,这是基于BeZnO的自供电紫外光电探测器的第一份报告。我们的发现证明了一种新颖且便捷的途径,可以实现用于多种用途的高性能自供电紫外线光电探测器。

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