Catalytic Asymmetric Dearomatizing Redox Cross Coupling of Ketones with Aryl Hydrazines Giving 1,4-Diketones

Shenlin Huang; Lisa Koetzner; Chandra Kanta De; Benjamin List

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Catalytic Asymmetric Dearomatizing Redox Cross Coupling of Ketones with Aryl Hydrazines Giving 1,4-Diketones

机译：酮与1,4-二酮的芳基肼催化不对称脱芳香化氧化还原交叉偶联

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摘要

An asymmetric Bronsted acid catalyzed dearomatizing redox cross coupling reaction has been realized, in which aryl hydrazines react with ketones to deliver 1,4-diketones, bearing an all-carbon quarternary stereocenter in high enantiopurity.

机译：已经实现了不对称的布朗斯台德酸催化的脱芳香化氧化还原交叉偶联反应，其中芳基肼与酮反应生成1,4-二酮，并带有高纯度的全碳四元立体中心。

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《Journal of the American Chemical Society》 |2015年第10期|3446-3449|共4页
作者
Shenlin Huang; Lisa Koetzner; Chandra Kanta De; Benjamin List;
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作者单位

Max-Planck-Institut fuer Kohlenforschung, Kaiser-Wilhelm-Platz 1, D-45470 Muelheim an der Ruhr, Germany;

Max-Planck-Institut fuer Kohlenforschung, Kaiser-Wilhelm-Platz 1, D-45470 Muelheim an der Ruhr, Germany;

Max-Planck-Institut fuer Kohlenforschung, Kaiser-Wilhelm-Platz 1, D-45470 Muelheim an der Ruhr, Germany;

Max-Planck-Institut fuer Kohlenforschung, Kaiser-Wilhelm-Platz 1, D-45470 Muelheim an der Ruhr, Germany;

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收录信息美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
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1. Cross-coupling of dissimilar ketone enolates via enolonium species to afford non-symmetrical 1,4-diketones [J] . Keshaba N. Parida, Gulab K. Pathe, Shimon Maksymenko, Beilstein journal of organic chemistry. . 2018,第1期

机译：通过en烯物种将异种酮烯酸酯交叉偶联以提供非对称的1,4-二酮
2. Formation of Unsymmetrical 1,4-Enediones via A Focusing Domino Strategy: Cross-Coupling of 1,3-Dicarbonyl Compounds and Methyl Ketones or Terminal Aryl Alkenes [J] . Gao M, Yang Y, Wu YD, Organic letters . 2010,第8期

机译：通过重点多米诺骨牌战略形成不对称的1,4-烯酮：1,3-二羰基化合物与甲基酮或末端芳烃的交叉偶联
3. Copper-Catalyzed Asymmetric Oxidative Cross-Coupling of 2-Naphthols with Aryl Methyl Ketones [J] . Deng Tao, Wang Hongjun, Cai Chun European journal of organic chemistry . 2015,第7期

机译：铜催化2-萘酚与芳基甲基酮的不对称氧化交叉偶联
4. Catalytic 1,4-Reduction of alpha,beta-Unsaturated Ketones and Application to Asymmetric Synthesis of Warfarin [C] . Yasunori Tsuchiya, Ken-ichi Moriya, Christine Beemelmanns Symposium on Organometallic Chemistry . 2006

机译：催化1,4-减少α，β-不饱和酮和施用于Warfarin的不对称合成
5. I. Abstraction of deuterium from dideuteroglycine by aryl radical: A model for 1,4-aryl diradical reactions with proteins. II. Acyl hydrazines as precursors to acyl radicals: Direct trapping and cyclization studies. [D] . Anderson, Marc Oliver. 2001

机译：I.通过芳基从双去氢甘氨酸提取氘：与蛋白质的1，4-芳基双自由基反应的模型。二。酰基肼作为酰基自由基的前体：直接捕获和环化研究。
6. Cross-coupling of dissimilar ketone enolates via enolonium species to afford non-symmetrical 14-diketones [O] . Keshaba N Parida, Gulab K Pathe, Shimon Maksymenko, 2018

机译：通过en烯物种将异种酮烯酸酯交叉偶联以提供非对称的14-二酮
7. Catalytic Asymmetric Reductive Acyl Cross-Coupling: Synthesis of Enantioenriched Acyclic α,α-Disubstituted Ketones [O] . Cherney Alan H., Kadunce Nathaniel T., Reisman Sarah E. 2013

机译：催化不对称还原性酰基交叉偶联：对映体富集的无环α，α-二取代酮的合成

Catalytic Asymmetric Dearomatizing Redox Cross Coupling of Ketones with Aryl Hydrazines Giving 1,4-Diketones

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