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Hydrogenated TiO2 nanobelts as highly efficient photocatalytic organic dye degradation and hydrogen evolution photocatalyst

机译:氢化TiO2纳米带作为高效的光催化有机染料降解和析氢光催化剂

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摘要

TiO2 nanobelts have gained increasing interest because of its outstanding properties and promising applications in a wide range of fields. Here we report the facile synthesis of hydrogenated TiO2 (H-TiO2) nanobelts, which exhibit excellent UV and visible photocatalytic decomposing of methyl orange (MO) and water splitting for hydrogen production. The improved photocatalytic property can be attributed to the Ti3+ ions and oxygen vacancies in TiO2 nanobelts created by hydrogenation. Ti3+ ions and oxygen vacancies can enhance visible light absorption, promote charge carrier trapping, and hinder the photogenerated electron-hole recombination. This work offers a simple strategy for the fabrication of a wide solar spectrum of active photocatalysts, which possesses significant potential for more efficient photodegradation, photocatalytic water splitting, and enhanced solar cells using sunlight as light source. (C) 2015 Elsevier B.V. All rights reserved.
机译:TiO2纳米带由于其出色的性能和在广泛领域中的应用前景而引起了越来越多的兴趣。在这里,我们报告氢化的TiO2(H-TiO2)纳米带的合成很容易,该纳米带表现出优异的UV和可见光催化分解的甲基橙(MO)以及水分解产生氢。改善的光催化性能可归因于由氢化产生的TiO2纳米带中的Ti3 +离子和氧空位。 Ti3 +离子和氧空位可增强可见光吸收,促进电荷载流子俘获并阻碍光生电子-空穴复合。这项工作为制造广谱的活性光催化剂提供了一种简单的策略,它具有利用日光作为光源进行更有效的光降解,光催化水分解和增强太阳能电池的巨大潜力。 (C)2015 Elsevier B.V.保留所有权利。

著录项

  • 来源
    《Journal of Hazardous Materials》 |2015年第15期|165-173|共9页
  • 作者单位

    Shandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R China|Shandong Univ, State Key Lab Crystal Mat, Jinan 250100, Peoples R China;

    Shandong Univ, State Key Lab Crystal Mat, Jinan 250100, Peoples R China;

    Shandong Univ Sci & Technol, Sch Mat Sci & Engn, Qingdao 266590, Peoples R China;

    Shandong Univ, State Key Lab Crystal Mat, Jinan 250100, Peoples R China;

  • 收录信息 美国《科学引文索引》(SCI);美国《工程索引》(EI);美国《生物学医学文摘》(MEDLINE);美国《化学文摘》(CA);
  • 原文格式 PDF
  • 正文语种 eng
  • 中图分类
  • 关键词

    Hydrogenation; TiO2 nanobelts; Photocatalytic; Hydrogen production; UV-visible;

    机译:加氢TiO2纳米带光催化制氢紫外可见;

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