OBT/HTO ratio in agricultural produce subject to routine atmospheric releases of tritium

摘要

The mean expected value of the OBT/HTO ratio (i.e. generic ratio) is derived in this study on the joint basis of a long-term study conducted at Atomic Energy of Canada Limited (AECL)'s Chalk River Laboratories (CRL), model simulations targeted at filling gaps in a yet incomplete timeline of CRL measurements and a reference dataset comprised of numerous experiments reported in the literature. Cultivar variability and disparity in site-specific settings are covered by the reference dataset. Dynamical variability caused by meteorology has been a specific target of the long-term experimental campaign at CRL, where the former two types of variability were eliminated. The distribution of OBT/HTO ratios observed at CRL appears to be a fairly good match to the distribution of OBT/HTO ratios from the literature. This implies that dynamical variability appears important in both cases. Dynamics of atmospheric HTO at CRL is comprised of a sequence of episodes of atmospheric HTO uptake and re-emission of plant HTO. The OBT/ HTO ratio appears sensitive to the proportion of the duration of these two episodes: the lesser the frequency (and duration) of plume arrivals, the higher the expected mean OBT/HTO ratio. With the plume arrival frequency defined by the typical wind rose, one would encounter a mean OBT/HTO ratio close to 2. It is important to note that this number is seen both in the reference dataset, and in the continuous timeline of HTO and OBT reconstructed from CRL observations by dynamical interpolation (modelling). Many datasets (including that of CRL) targeted at the OBT/HTO ratio are biased high compared to the suggested number. This could be explained by scarce measurements of the low OBT/ HTO ratios in the short phase of uptake of atmospheric HTO by the plant.