Impact of the anode operating conditions on the liquid water distribution in the cathode gas diffusion layer

摘要

Previous experimental results indicate that the humidification conditions at the anode have an impact on the liquid water distribution in the cathode gas diffusion layer. Numerical simulations are developed to reproduce and analyze this effect. Results consistent with the experimental results are first obtained by playing with the partition coefficients of an advanced pore network model computing the liquid water formation and transfer in the cathode gas diffusion layer (GDL) for a large range of operating conditions. Then, a model for the full anode - cathode assembly is developed by combining the pore network model of the cathode GDL and a 1D model describing the heat and water transfer in the various components of the anode-cathode assembly. This enables one to generalize the dry - wet regime diagram introduced in a previous work by incorporating the effect of the humidity condition at the anode.(c)& nbsp;2020 Hydrogen Energy Publications LLC. Published by Elsevier Ltd. All rights reserved.