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Nuclear Resonance Fluorescence for Materials Assay

机译:核共振荧光分析

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摘要

This paper discusses the use of nuclear resonance fluorescence (NRF) techniques for the isotopic and quantitative assaying of radioactive material. Potential applications include age-dating of an unknown radioactive source, pre- and post-detonation nuclear forensics and safeguards for nuclear fuel cycles Examples of age-dating a strong radioactive source and assaying a spent fuel pin are discussed. The modeling work has ben performed with the Monte Carlo radiation transport computer code MCNPX and the capability to simulate NRF has bee added to the code. Discussed are the limitations in MCNPX's photon transport physics for accurately describing photon scattering processes that are important contributions to the background and impact the applicability of the NRF assay technique.
机译:本文讨论了使用核磁共振荧光(NRF)技术进行放射性物质的同位素和定量测定。潜在的应用包括未知放射性源的年代测定,爆炸前和爆炸后的核法证以及核燃料循环的保障措施。讨论了对强放射性源进行年代测定和分析乏燃料销的实例。已经使用蒙特卡罗辐射传输计算机代码MCNPX进行了建模工作,并且在代码中添加了模拟NRF的功能。讨论了MCNPX的光子传输物理学在准确描述光子散射过程方面的局限性,这些局限性是对背景的重要贡献,并影响NRF分析技术的适用性。

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