Time Response of the Lake Ontario Ecosystem to Virtual Elimination of PCBs

摘要

This study presents the development, application, and partial validation of an integrated time-dependent whole ecosystem environmental fate and food-chain bioaccumulation model of the time response of PCB concentrations in various media and organisms of Lake Ontario to changes in external PCB loadings to the lake. The model and observed PCB concentration time trends in herring gull eggs, lake trout, sculpins, smelt, water, and sediment data are used to reconstruct the time response and PCB loading history for Lake Ontario and to assess the past and future time response of PCB concentrations in the Lake Ontario food web to PCB inputs. Estimates of loadings, concentrations, half-lifetimes, and changes in PCB composition over time are discussed.