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首页> 外文期刊>Npj Climate and Atmospheric Science >Stochastic nucleation processes and substrate abundance explain time-dependent freezing in supercooled droplets
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Stochastic nucleation processes and substrate abundance explain time-dependent freezing in supercooled droplets

机译:随机成核过程和底物丰度解释过冷却液滴中的时间依赖性冻结

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Atmospheric immersion freezing (IF), a heterogeneous ice nucleation process where an ice nucleating particle (INP) is immersed in supercooled water, is a dominant ice formation pathway impacting the hydrological cycle and climate. Implementation of IF derived from field and laboratory data in cloud and climate models is difficult due to the high variability in spatio-temporal scales, INP composition, and morphological complexity. We demonstrate that IF can be consistently described by a stochastic nucleation process accounting for uncertainties in the INP surface area. This approach accounts for time-dependent freezing, a wide range of surface areas and challenges phenomenological descriptions typically used to interpret IF. The results have an immediate impact on the current description, interpretation, and experiments of IF and its implementation in models. The findings are in accord with nucleation theory, and thus should hold for any supercooled liquid material that nucleates in contact with a substrate.
机译:大气浸没冷冻(IF),浸入过冷水中浸入冰核颗粒(INP)的异质冰成核过程,是影响水文循环和气候的主要冰形成途径。由于时空尺度,INP成分和形态复杂性的高度变化,如果云和气候模型中的云和气候模型中源于云和气候模型的实验室数据的实施。我们证明,如果可以通过随机成核过程一致地描述在INP表面积中的不确定性。这种方法考虑了时间依赖的冻结,范围广泛的表面积和挑战通常用于解释的现象学描述。结果对模型中的当前描述,解释和实验产生了立即影响。结果符合成核理论,因此应保持任何与基材接触的过脱液液体材料。

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