Origin, Maintenance and Variability of the Asian Tropopause Aerosol Layer (ATAL): The Roles of Monsoon Dynamics

摘要

Using NASA MERRA2 daily data, we investigated the origin, maintenance and variability of the Asian Tropopause Aerosol Layer (ATAL) in relation to variations of the Asia Monsoon Anticyclone (AMA) during the summer of 2008. During May-June, abundant quantities of carbon monoxide (CO), carbonaceous aerosols (CA) and dusts are found in the mid- and upper troposphere over India and China, arising from enhanced biomass burning emissions, as well as westerly transport from the Middle East deserts. During July-August, large quantities of dusts transported from the deserts are trapped and accumulate over the southern and eastern foothills of the Tibetan Plateau. Despite strong precipitation washout, ambient CO, CA and dust are lofted by orographically forced deep convection to great elevations, 12–16?km above sea level, via two key pathways over heavily polluted regions: a) the Himalayas-Gangetic Plain, and b) the Sichuan Basin. Upon entering the upper-troposphere-lower-stratosphere, the pollutants are capped by a stable layer near the tropopause, advected and dispersed by the anticyclonic circulation of AMA, forming the ATAL resembling a planetary-scale “double-stem chimney cloud”. The development and variability of the ATAL are strongly linked to the seasonal march and intraseasonal (20–30 days and higher frequency) oscillations of the Asian monsoon.