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One-step fabrication of crystalline metal nanostructures by direct nanoimprinting below melting temperatures

机译:在低于熔点的温度下通过直接纳米压印一步一步制造晶体金属纳米结构

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摘要

Controlled fabrication of metallic nanostructures plays a central role in much of modern science and technology, because changing the dimensions of a nanocrystal enables tailoring of its mechanical, electronic, optical, catalytic and antibacterial properties. Here we show direct superplastic nanoimprinting (SPNI) of crystalline metals well below their melting temperatures, generating ordered nanowire arrays with aspect ratios up to ~2,000 and imprinting features as small as 8?nm. Surface-enhanced Raman scattering (SERS) spectra reveal strongly enhanced electromagnetic signals from the prepared nanorod arrays with sizes up to ~100?nm, which indicates that our technique can provide an ideal way to fabricate robust SERS substrates. SPNI, as a one-step, controlled and reproducible nanofabrication method, could facilitate the applications of metal nanostructures in bio-sensing, diagnostic imaging, catalysis, food industry and environmental conservation.
机译:在许多现代科学和技术中,金属纳米结构的受控制造起着至关重要的作用,因为改变纳米晶体的尺寸可以对其机械,电子,光学,催化和抗菌性能进行定制。在这里,我们显示了远低于其熔融温度的结晶金属的直接超塑性纳米压印(SPNI),生成了纵横比高达2,000左右且压印特征小至8?nm的有序纳米线阵列。表面增强拉曼散射(SERS)光谱揭示了制备的纳米棒阵列的电磁信号大大增强,尺寸高达〜100?nm,这表明我们的技术可以为制造坚固的SERS基底提供理想的方法。 SPNI作为一种可控制的,可重复的纳米制造方法,可以促进金属纳米结构在生物传感,诊断成像,催化,食品工业和环境保护中的应用。

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