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A regional air quality forecasting system over Europe: the MACC-II daily ensemble production

机译:欧洲区域性空气质量预报系统:MACC-II每日整体产量

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This paper describes the pre-operational analysis and forecasting systemdeveloped during MACC (Monitoring Atmospheric Composition and Climate) andcontinued in the MACC-II (Monitoring Atmospheric Composition and Climate:Interim Implementation) European projects to provide air quality servicesfor the European continent. This system is based on seven state-of-the artmodels developed and run in Europe (CHIMERE, EMEP, EURAD-IM, LOTOS-EUROS,MATCH, MOCAGE and SILAM). These models are used to calculate multi-modelensemble products. The paper gives an overall picture of its status at theend of MACC-II (summer 2014) and analyses the performance of the multi-modelensemble. The MACC-II system provides daily 96 h forecasts with hourlyoutputs of 10 chemical species/aerosols (O3, NO2, SO2, CO,PM10, PM2.5, NO, NH3, total NMVOCs (non-methane volatile organic compounds) andPAN+PAN precursors) over eight vertical levels from the surface to 5 km height.The hourly analysis at the surface is done a posteriori for the past day using aselection of representative air quality data from European monitoringstations.The performance of the system is assessed daily, weekly and every 3 months(seasonally) through statistical indicators calculated using the availablerepresentative air quality data from European monitoring stations. Resultsfor a case study show the ability of the ensemble median to forecastregional ozone pollution events. The seasonal performances of the individualmodels and of the multi-model ensemble have been monitored since September2009 for ozone, NO2 and PM10. The statistical indicators for ozonein summer 2014 show that the ensemble median gives onaverage the best performances compared to the seven models. There is very little degradation ofthe scores with the forecast day but there is a marked diurnal cycle,similarly to the individual models, that can be related partly to theprescribed diurnal variations of anthropogenic emissions in the models.During summer 2014, the diurnal ozone maximum is underestimated by theensemble median by about 4 μg m?3 on average. Locally, during thestudied ozone episodes, the maxima from the ensemble median are often lowerthan observations by 30–50 μg m?3. Overall, ozone scores aregenerally good with average values for the normalised indicators of 0.14 forthe modified normalised mean bias and of 0.30 for the fractional grosserror. Tests have also shown that the ensemble median is robust to reductionof ensemble size by one, that is, if predictions are unavailable from onemodel. Scores are also discussed for PM10 for winter 2013–1014. Thereis an underestimation of most models leading the ensemble median to amean bias of ?4.5 μg m?3. The ensemble median fractional grosserror is larger for PM10 (~ 0.52) than for ozone andthe correlation is lower (~ 0.35 for PM10 and~ 0.54 for ozone). This is related to a larger spread of the sevenmodel scores for PM10 than for ozone linked to different levels ofcomplexity of aerosol representation in the individual models. In parallel,a scientific analysis of the results of the seven models and of the ensembleis also done over the Mediterranean area because of the specificity of itsmeteorology and emissions.The system is robust in terms of the production availability. Major effortshave been done in MACC-II towards the operationalisation of all itscomponents. Foreseen developments and research for improving itsperformances are discussed in the conclusion.
机译:本文介绍了在MACC(监测大气成分和气候)期间开发的,并在MACC-II(监测大气成分和气候:临时实施)欧洲项目中继续进行的运行前分析和预报系统,以为欧洲大陆提供空气质量服务。该系统基于在欧洲开发和运行的七个最新模型(CHIMERE,EMEP,EURAD-IM,LOTOS-EUROS,MATCH,MOCAGE和SILAM)。这些模型用于计算多模型集成产品。本文概述了MACC-II末期(2014年夏季)的状态,并分析了多模型集成的性能。 MACC-II系统每天提供96小时预报,每小时输出10种化学物质/气溶胶(O 3 ,NO 2 ,SO 2 ,CO ,PM 10 ,PM 2.5 ,NO,NH 3 ,总NMVOC(非甲烷挥发性有机化合物)和PAN + PAN前体从地面到5 km高的垂直高度。过去一天中,每小时的地面分析都是使用欧洲监测站提供的代表性空气质量数据进行后验的。 系统的性能每天进行评估,通过统计指标每周和每3个月(季节性)使用欧洲监测站提供的代表性空气质量数据进行计算。案例研究结果表明,集合中值能够预测区域臭氧污染事件。自2009年9月以来,已监测了各个模型和多模型集合的季节性表现,包括臭氧,NO 2 和PM 10 。 2014年夏季臭氧的统计指标表明,与七个模型相比,集合中值平均给出了最佳性能。与预报日相比,分数几乎没有降级,但有一个明显的昼夜周期,类似于各个模型,这可能部分与模型中人为排放的规定昼夜变化有关。2014年夏季,昼夜臭氧最大值为总体中位数低估了约4μgm ?3 。在当地,在研究的臭氧事件中,集合中值的最大值通常比观测值低30–50μgm ?3 。总体而言,臭氧得分总体而言是良好的,对于修正后的归一化平均偏差,归一化指标的平均值为0.14,对于分数总误差为0.30。测试还表明,合奏中位数对于将合奏大小减小1(即,如果无法从一个模型获得预测)具有鲁棒性。还讨论了2013-1014年冬季PM 10 的得分。大多数模型都低估了整个集合的中位数,从而使阿曼偏差为?4.5μgm ?3 。 PM 10 的整体中值部分总误差大于臭氧(〜0.52),并且相关性较低(PM 10 的〜0.35和臭氧约为0.54)。这与PM 10 的七个模型得分的散布相比于臭氧的散布有关,后者与各个模型中不同的气溶胶表示复杂度有关。同时,由于其气象学和排放的特殊性,还对地中海地区的七个模型和集合进行了科学分析。 该系统在生产可用性方面非常强大。 MACC-II在所有组件的操作方面已经做出了重大努力。结论中讨论了可预期的发展和改进其性能的研究。

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