COsub2/sub drawdown due to particle ballasting by glacial aeolian dust: an estimate based on the ocean carbon cycle model MPIOM/HAMOCC version 1.6.2p3

摘要

Despite intense efforts, the mechanisms that drive glacial–interglacial changes in atmospheric pCOsub2/sub are not fully understood. Here, we aim at quantifying the potential contribution of aeolian dust deposition changes to the atmospheric pCOsub2/sub drawdown during the Last Glacial Maximum (LGM). To this end, we use the Max Planck Institute Ocean Model (MPIOM) and the embedded Hamburg Ocean Carbon Cycle model (HAMOCC), including a new parameterization of particle ballasting that accounts for the acceleration of sinking organic soft tissue in the ocean by higher-density biogenic calcite and opal particles, as well as mineral dust. Sensitivity experiments with reconstructed LGM dust deposition rates indicate that the acceleration of detritus by mineral dust played a small role in atmospheric pCOsub2/sub variations during glacial–interglacial cycles – on the order of 5?ppmv, compared to the reconstructed ～80 ppmv rise in atmospheric pCOsub2/sub during the last deglaciation. The additional effect of the LGM dust deposition, namely the enhanced fertilization by the iron that is associated with the glacial dust, likely played a more important role; although the full iron fertilization effect can not be estimated in the particular model version used here due to underestimated present-day non-diazotroph iron limitation, fertilization of diazotrophs in the tropical Pacific already leads to an atmospheric pCOsub2/sub drawdown of around 10?ppmv.