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Characterization of uncertainties in atmospheric trace gas inversions using hierarchical Bayesian methods

机译:使用分级贝叶斯方法表征大气痕量气体反演中的不确定性

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pstrongAbstract./strong We present a hierarchical Bayesian method for atmospheric trace gas inversions. This method is used to estimate emissions of trace gases as well as "hyper-parameters" that characterize the probability density functions (PDFs) of the a priori emissions and model-measurement covariances. By exploring the space of "uncertainties in uncertainties", we show that the hierarchical method results in a more complete estimation of emissions and their uncertainties than traditional Bayesian inversions, which rely heavily on expert judgment. We present an analysis that shows the effect of including hyper-parameters, which are themselves informed by the data, and show that this method can serve to reduce the effect of errors in assumptions made about the a priori emissions and model-measurement uncertainties. We then apply this method to the estimation of sulfur hexafluoride (SFsub6/sub) emissions over 2012 for the regions surrounding four Advanced Global Atmospheric Gases Experiment (AGAGE) stations. We find that improper accounting of model representation uncertainties, in particular, can lead to the derivation of emissions and associated uncertainties that are unrealistic and show that those derived using the hierarchical method are likely to be more representative of the true uncertainties in the system. We demonstrate through this SFsub6/sub case study that this method is less sensitive to outliers in the data and to subjective assumptions about a priori emissions and model-measurement uncertainties than traditional methods./p.
机译:> >摘要。我们提出了一种用于大气痕量气体反演的分层贝叶斯方法。此方法用于估计痕量气体的排放以及表征先验排放和模型测量协方差的概率密度函数(PDF)的“超参数”。通过探索“不确定性的不确定性”空间,我们表明,与传统的贝叶斯反演方法相比,分层方法可以更全面地估算排放量及其不确定性,而传统的贝叶斯反演方法严重依赖专家的判断。我们提出了一项分析,该分析表明了包括超参数的影响,而超参数本身是由数据告知的,并且表明,该方法可以减少对先验排放和模型测量不确定性所作的假设中的误差影响。然后,我们将该方法用于估算四个全球高级大气实验站(AGAGE)周围地区2012年的六氟化硫(SF 6 )排放。我们发现,模型表示不确定性的不正确计算尤其会导致排放和相关不确定性的推导,这些推导是不现实的,并表明使用分层方法得出的不确定性可能更能代表系统中的真实不确定性。我们通过SF 6 案例研究证明,该方法比传统方法对数据中的异常值以及对先验排放和模型测量不确定性的主观假设不太敏感。

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