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Quantifying pollution transport from the Asian monsoon anticyclone into the lower stratosphere

机译:量化从亚洲季风反气旋到平流层下层的污染输送

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Pollution transport from the surface to the stratosphere within the Asian monsoon circulation may cause harmful effects on stratospheric chemistry and climate. Here, we investigate air mass transport from the monsoon anticyclone into the stratosphere using a Lagrangian chemistry transport model. We show how two main transport pathways from the anticyclone emerge: (i)?into the tropical stratosphere (tropical pipe), and (ii)?into the Northern Hemisphere (NH) extratropical lower stratosphere. Maximum anticyclone air mass fractions reach around 5?% in the tropical pipe and 15?% in the extratropical lowermost stratosphere over the course of a year. The anticyclone air mass fraction correlates well with satellite hydrogen cyanide (HCN) and carbon monoxide (CO) observations, confirming that pollution is transported deep into the tropical stratosphere from the Asian monsoon anticyclone. Cross-tropopause transport occurs in a vertical chimney, but with the pollutants transported quasi-horizontally along isentropes above the tropopause into the tropics and NH.
机译:在亚洲季风环流中,污染物从地表到平流层的迁移可能对平流层的化学和气候产生有害影响。在这里,我们使用拉格朗日化学迁移模型研究了从季风反气旋进入平流层的空气质量迁移。我们展示了如何从反气旋产生两种主要的运输途径:(i)进入热带平流层(热带管道),和(ii)进入北半球(NH)温带下层平流层。在一年的时间里,热带管道中最大的反气旋空气质量分数达到5%左右,而温带最低的平流层中则达到15 %%。反气旋空气质量分数与卫星氰化氢(HCN)和一氧化碳(CO)观测值密切相关,这证实了污染物是从亚洲季风反气旋深入到热带平流层的。跨对流层顶运输发生在垂直烟囱中,但是污染物沿对流层顶上方的等熵线准水平地运输到热带和NH。

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