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Enhanced photocatalytic H2 evolution over CdS/Au/g-C3N4 composite photocatalyst under visible-light irradiation

机译:在可见光照射下,CdS / Au / g-C3N4复合光催化剂的光催化氢气释放增强

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A novel heterojunction structured composite photocatalyst CdS/Au/g-C3N4 has been developed by depositing CdS/Au with a core (Au)-shell (CdS) structure on the surface of g-C3N4. The photocatalytic hydrogen production activity of the developed photocatalyst was evaluated under visible-light irradiation (λ > 420 nm) using methanol as a sacrificial reagent. As a result, its activity is about 125.8 times higher than that of g-C3N4 and is even much higher than that of Pt/g-C3N4. The enhancement in photocatalytic activity is attributed to efficient separation of the photoexcited charges due to the anisotropic junction in the CdS/Au/g-C3N4 system.
机译:通过在g-C3N4表面沉积具有核心(Au)-壳(CdS)结构的CdS / Au,开发了一种新型的异质结结构复合光催化剂CdS / Au / g-C3N4。使用甲醇作为牺牲剂,在可见光照射下(λ> 420 nm)评估显影后的光催化剂的光催化产氢活性。结果,其活性比g-C3N4高约125.8倍,甚至比Pt / g-C3N4高得多。由于CdS / Au / g-C3N4系统中的各向异性结,光催化活性的提高归因于光激发电荷的有效分离。

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