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Investigations of mass transfer in annular gas-liquid flow in a microreactor

机译:微反应器中环形气液流动中传质的研究

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The paper presents an investigation of mass transfer in gas-liquid annular flow in a microreactor. The microreactor had a meandered shape with a square cross-section of the channel (292×292 μm, hydraulic diameter 292 μm) and 250 mm in length. The rate of CO2 absorption from the CO2/N2 mixture in NaOH (0.1 M, 0.2 M, 0.7 M, 1.0 M and 1.5 M) water solutions was measured. Two velocities of gas flow and two velocities of liquid flow were used. In two cases a fully developed annular flow at the beginning of the channel was observed, whilst in two cases annular flow was formed only in about 2/3 of the microchannel length. Based on the measurements of CO2 absorption rate, the values of volumetric liquid - side mass transfer coefficients with the chemical reaction were determined. Then physical values of coefficients were found. Obtained results were discussed and their values were compared with the values predicted by literature correlations.
机译:本文介绍了在微反应器中气液环流中传质的研究。微反应器呈曲折形状,其通道的横截面为正方形(292×292μm,水力直径292μm),长度为250 mm。测量了在NaOH(0.1 M,0.2 M,0.7 M,1.0 M和1.5 M)水溶液中从CO2 / N2混合物吸收CO2的速率。使用两种流速的气体流速和两种流速的液体流速。在两种情况下,观察到在通道开始处完全形成的环形流,而在两种情况下,仅在微通道长度的约2/3处形成环形流。基于对CO 2吸收率的测量,确定了伴随化学反应的液体-质量侧传质系数的值。然后找到系数的物理值。对获得的结果进行了讨论,并将其值与文献相关性预测的值进行了比较。

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