Occurrence and fate of antibiotics and heavy metals in sewage treatment plants and risk assessment of reclaimed water in Chengdu, China

摘要

Aim of this study was to provide an up-to-date assessment of the heavy metals and antibiotics in reclaimed water in Chengdu, China. 3 sewage treatment plants (STPs) and 1 constructed wetland (CW) were first taken as the research objects. The total concentration and reduction change rule of heavy metals and antibiotics in the process of reclaimed water production were investigated. The possible health risks to ecological environment and human body were evaluated. For the treatment process, the Cyclic Activated Sludge System (CASS) used in A sewage treatment plant (STP A) had the best removal effect for heavy metals. When the proportion of industrial wastewater in the influent was relatively high, the heavy metal pollution level was alert. Ofloxacin (OFX) and roxithromycin (ROX) were the most abundant antibiotics in reclaimed water. After being removed by the sewage treatment system, OFX concentrations changed, but several of them remained in reclaimed water. Negative removal of ROX occurred. This is because macrolides were wrapped in human feces, whose concentration increased as feces disperse and hydrolyze. Compared with CASS (20.02%) and Anaerobic-Anoxic-Oxic process (A(2)/O 34.16%), the average removal rate of antibiotics from the A(2)/O accompanied by Membrane Bio-Reactor (71.1%) and CW (54.95%) was higher. When the proportion of domestic sewage in wastewater was high, antibiotics in reclaimed water had higher ecological risk. OFX had the highest ecological risk for non-target aquatic organisms. It was assessed that the heavy metals and antibiotics studied did not pose a carcinogenic or non-carcinogenic risk to human health. (C) 2021 Elsevier Ltd. All rights reserved.