Growth of Crystalline Polyaminoborane through Catalytic Dehydrogenation of Ammonia Borane on FeB Nanoalloy

Teng He; Prof. Junhu Wang; Dr. Guotao Wu; Dr. Hyunjeong Kim; Dr. Thomas Proffen; Dr. Anan Wu; Wen Li; Tao Liu; Prof. Zhitao Xiong; Dr. Chengzhang Wu; Dr. Hailiang Chu; Jianping Guo; Dr. Tom Autrey; Prof. Tao Zhang; Prof. Ping Chen

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Growth of Crystalline Polyaminoborane through Catalytic Dehydrogenation of Ammonia Borane on FeB Nanoalloy

机译：FeB纳米合金上氨硼烷的催化脱氢生长结晶型聚氨基硼烷

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Nano-alloy: Crystalline polyaminoborane is formed upon releasing 1.0 equivalent H₂ from ammonia borane at 60 °C catalyzed by a nano-FeB alloy. Our experimental results show that about 1.0 and 1.5 equiv H₂ can be released at 60 and 100 °C, respectively.

机译：纳米合金：在60°C下由纳米FeB合金催化从氨硼烷中释放1.0当量的H _{2 形成结晶聚氨基硼烷。我们的实验结果表明，分别在60和100 C下可以释放约1.0和1.5 equiv H _{2 。}}

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来源
《Chemistry - A European Journal》 |2010年第43期|p.12814-12817|共4页
作者
Teng He; Prof. Junhu Wang; Dr. Guotao Wu; Dr. Hyunjeong Kim; Dr. Thomas Proffen; Dr. Anan Wu; Wen Li; Tao Liu; Prof. Zhitao Xiong; Dr. Chengzhang Wu; Dr. Hailiang Chu; Jianping Guo; Dr. Tom Autrey; Prof. Tao Zhang; Prof. Ping Chen;
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作者单位

Dalian Institute of Chemical Physics, Chinese Academy of Sciences, 457# Zhongshan Road, 116023 Dalian (China), Fax: (+86)

411-84685940;

Lujan Neutron Scattering Center, Los Alamos National Laboratory, Los Alamos, New Mexico, 87545 (USA);

State Key laboratory of Physical Chemical of Solid Surfaces, Xiamen University, YanWu Road, Xiamen, Fujian, 361005 (China);

Department of Physics, National University of Singapore, 10 Kent Ridge Crescent, 117542 (Singapore);

Institute for Synchrotron Radiation, Karlsruhe Institute of Technology, 76344 Karlsruhe (Germany);

Pacific Northwest National Laboratory, Richland, WA 99352 (USA);

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正文语种 eng
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关键词
alloys; boranes; dehydrogenation; heterogeneous catalysis; nanoalloy;

机译：合金;硼烷;脱氢;非均相催化;纳米合金;

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专利

1. Growth of crystalline polyaminoborane through catalytic dehydrogenation of ammonia borane on FeB nanoalloy [J] . He T., Wang J., Wu G., Chemistry: A European journal . 2010,第43期

机译：FeB纳米合金上氨硼烷催化脱氢生长结晶聚氨基硼烷
2. Quasi in situ Mossbauer and XAS studies on FeB nanoalloy for heterogeneous catalytic dehydrogenation of ammonia borane [J] . Teng He, Junhu Wang, Tao Liu Catalysis Today . 2011,第1期

机译：FeB纳米合金用于氨硼烷非均相催化脱氢的准原位Mossbauer和XAS研究
3. Catalytic Dehydrocoupling/Dehydrogenation of N-Methylamine-Borane and Ammonia-Borane: Synthesis and Characterization of High Molecular Weight Polyaminoboranes [J] . Anne Staubitz, Matthew E. Sloan, Alasdair P. M. Robertson, Journal of the American Chemical Society . 2010,第38期

机译：N-甲胺-硼烷和氨-硼烷的催化脱氢偶联/脱氢：高分子量聚氨基硼烷的合成与表征
4. Fabrication of Hollow Silica-alumina Composite Spheres Using L(+)-arginine and Their Catalytic Performance for Hycfrolytic Dehydrogenation of Ammonia Borane [C] . Tetsuo Umeqaki, Shunsuke Imamura, Naoki Toyama International Symposium on Inorganic Environmental Materials . 2014

机译：使用L（+） - 精氨酸 - 精氨酸的中空二氧化硅 - 氧化铝复合球的制备及其催化性能，对氨硼烷的Hycfrolytic脱氢
5. Catalytic Dehydrogenation of Ammonia Borane-Polyvinylpyrrolidone Hydrogen Storage Composites with Different Molecular Weights [D] . Seemaladinne, Ramanjaneyulu. 2017

机译：不同分子量氨硼烷-聚乙烯基吡咯烷酮储氢复合材料的催化脱氢
6. Probing the second dehydrogenation step in ammonia-borane dehydrocoupling: characterization and reactivity of the key intermediate B-(cyclotriborazanyl)amine-borane [O] . Hassan A. Kalviri, Felix Gärtner, Gang Ye, 2015

机译：探索氨-硼烷脱氢偶联反应中的第二个脱氢步骤：关键中间体B-（环三氮杂硼烷基）胺-硼烷的表征和反应性
7. Growth of Crystalline Polyaminoborane through Catalytic Dehydrogenation of Ammonia Borane on FeB Nanoalloy [O] . He Teng ( Chinese Acad Sci Dalian Inst Chem Phys Dalian), Wang Junhu ( Chinese Acad Sci Dalian Inst Chem Phys Dalian), Wu Guotao ( Chinese Acad Sci Dalian Inst Chem Phys Dalian), 2010

机译：FeB纳米合金上氨硼烷的催化脱氢生长结晶型聚氨基硼烷

Growth of Crystalline Polyaminoborane through Catalytic Dehydrogenation of Ammonia Borane on FeB Nanoalloy

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