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Chemical and photochemical oxidation of organic substrates by ruthenium aqua complexes with water as an oxygen source

机译：钌-水配合物以水为氧源对有机底物进行化学和光化学氧化

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摘要

Two ruthenium aqua complexes were shown to be effective catalysts in chemical and photochemical oxidation of hydrocarbons. A remarkable activity (up to 90% yield and 100% selectivity) was performed in conversion of sulfide to sulfoxide by homogeneous photooxidation. In Photosystem II (PSII), water is oxidized by sunlight with the oxygen-evolving complex (OEC) providing electrons and protons for sustainable processes in nature.
机译：两种钌水配合物被证明是烃类化学和光化学氧化的有效催化剂。通过均相光氧化将硫化物转化为亚砜时，具有显着的活性（高达90％的收率和100％的选择性）。在光系统II（PSII）中，水被太阳光与放氧复合物（OEC）氧化，从而为自然界的可持续过程提供电子和质子。

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  • 来源
    《Chemical Communications》 |2011年第31期|p.8949-8951|共3页
  • 作者

    Fei Li; Miao Yu; Yi Jiang; Fang Huang; Yanqing Li; Biaobiao Zhang; Licheng Sun;

  • 作者单位

    State Key Laboratory of Fine Chemicals, Dalian University of Technology (DVT), DUT-KTH Joint Education and Research Center on Molecular Devices, Dalian 116024, China;

    State Key Laboratory of Fine Chemicals, Dalian University of Technology (DVT), DUT-KTH Joint Education and Research Center on Molecular Devices, Dalian 116024, China;

    State Key Laboratory of Fine Chemicals, Dalian University of Technology (DVT), DUT-KTH Joint Education and Research Center on Molecular Devices, Dalian 116024, China;

    State Key Laboratory of Fine Chemicals, Dalian University of Technology (DVT), DUT-KTH Joint Education and Research Center on Molecular Devices, Dalian 116024, China;

    State Key Laboratory of Fine Chemicals, Dalian University of Technology (DVT), DUT-KTH Joint Education and Research Center on Molecular Devices, Dalian 116024, China;

    State Key Laboratory of Fine Chemicals, Dalian University of Technology (DVT), DUT-KTH Joint Education and Research Center on Molecular Devices, Dalian 116024, China;

    State Key Laboratory of Fine Chemicals, Dalian University of Technology (DVT), DUT-KTH Joint Education and Research Center on Molecular Devices, Dalian 116024, China,Department of Chemistry, School of Chemical Science and Engineering, Royal Institute of Technology (KTH), 100 44 Stockholm, Sweden;

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  • 入库时间 2022-08-17 13:22:42

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