Catalytic hydrogen production by a Ni-Ru mimic of NiFe hydrogenases involves a proton-coupled electron transfer step

Sigolene Canaguier; Vincent Fourmond; Carlo U. Perotto; Jennifer Fize; Jacques Pecaut; Marc Fontecave; Martin J. Field; Vincent Artero

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Catalytic hydrogen production by a Ni-Ru mimic of NiFe hydrogenases involves a proton-coupled electron transfer step

机译：NiFe氢化酶的Ni-Ru模拟产生催化氢涉及质子耦合电子转移步骤

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A combined electrochemical and theoretical study suggests that hydrogen evolution from weak acids catalyzed by a structural mimic of the active site of NiFe hydrogenases [Ni(xbsms)Ru(C_6Me_6)Cl]~+ proceeds through proton-coupled electron transfer steps.

机译：电化学和理论相结合的研究表明，NiFe加氢酶[Ni（xbsms）Ru（C_6Me_6）Cl]〜+的活性位点的结构模拟可催化弱酸中的氢释放，通过质子偶联电子转移步骤进行。

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来源
《Chemical Communications》 |2013年第44期|5004-5006|共3页
作者
Sigolene Canaguier; Vincent Fourmond; Carlo U. Perotto; Jennifer Fize; Jacques Pecaut; Marc Fontecave; Martin J. Field; Vincent Artero;
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Laboratoire de Chimie et Biologie des Metaux, Universite Joseph Fourier, Grenoble, France,CNRS, UMR 5249, France,CEA, DSV/iRTSV, 17 rue des Martyrs, F-38054 Grenoble Cedex 9, France;

Laboratoire de Chimie et Biologie des Metaux, Universite Joseph Fourier, Grenoble, France,CNRS, UMR 5249, France,CEA, DSV/iRTSV, 17 rue des Martyrs, F-38054 Grenoble Cedex 9, France ,Laboratoire de Bioenergetique et ingenierie des proteines, UMR 7281 CNRS-AMU, 31 chemin joseph Aiguier, 13402 Marseille, France;

Laboratoire de Chimie et Biologie des Metaux, Universite Joseph Fourier, Grenoble, France,CNRS, UMR 5249, France,CEA, DSV/iRTSV, 17 rue des Martyrs, F-38054 Grenoble Cedex 9, France ,DYNAMO/DYNAMOP, Institut de Biologie Structurale "Jean-Pierre Ebel", UMR CNRS/Universite Joseph Fourier/CEA 5075, 41 rue Jules Horowitz, F-38027 Grenoble Cedex 1, France;

Laboratoire de Chimie et Biologie des Metaux, Universite Joseph Fourier, Grenoble, France,CNRS, UMR 5249, France,CEA, DSV/iRTSV, 17 rue des Martyrs, F-38054 Grenoble Cedex 9, France;

Laboratoire de Reconnaissance Ionique et Chimie de Coordination, UMR-E3 Universite Joseph Fourier/CEA, 17 rue des Martyrs, F-38054 Grenoble Cedex 9, France;

Laboratoire de Chimie et Biologie des Metaux, Universite Joseph Fourier, Grenoble, France,CNRS, UMR 5249, France,CEA, DSV/iRTSV, 17 rue des Martyrs, F-38054 Grenoble Cedex 9, France ,College de France, 11 place Marcellin Berthelot, 75005 Paris, France;

DYNAMO/DYNAMOP, Institut de Biologie Structurale "Jean-Pierre Ebel", UMR CNRS/Universite Joseph Fourier/CEA 5075, 41 rue Jules Horowitz, F-38027 Grenoble Cedex 1, France;

Laboratoire de Chimie et Biologie des Metaux, Universite Joseph Fourier, Grenoble, France,CNRS, UMR 5249, France,CEA, DSV/iRTSV, 17 rue des Martyrs, F-38054 Grenoble Cedex 9, France;

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入库时间 2022-08-17 13:18:21

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机译：谷氨酸门控质子偶联电子转移活性niFe - 氢酶

Catalytic hydrogen production by a Ni-Ru mimic of NiFe hydrogenases involves a proton-coupled electron transfer step

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