Rhodium(Ⅱ)-catalysed tandem aziridination and ring-opening: stereoselective synthesis of functionalised tetrahydrofurans

William P. Unsworth; Nicola Clark; Thomas O. Ronson; Kiri Stevens; Amber L. Thompson; Scott G. Lamont; Jeremy Robertson

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Rhodium(Ⅱ)-catalysed tandem aziridination and ring-opening: stereoselective synthesis of functionalised tetrahydrofurans

机译：铑（Ⅱ）催化串联叠氮化和开环：功能化四氢呋喃的立体选择性合成

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摘要

Aziridines formed upon treatment of allylic carbamates and homo-allylic sulfamates with Rh(Ⅱ) carboxylate catalysts under oxidative conditions are trapped by suitably-disposed hydroxyl groups to give functionalised tetrahydrofurans.

机译：在氧化条件下用Rh（Ⅱ）羧酸盐催化剂处理烯丙基氨基甲酸酯和均烯丙基氨基磺酸酯后形成的氮丙啶被适当分布的羟基捕获，得到官能化的四氢呋喃。

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《Chemical Communications》 |2014年第77期|11393-11396|共4页
作者
William P. Unsworth; Nicola Clark; Thomas O. Ronson; Kiri Stevens; Amber L. Thompson; Scott G. Lamont; Jeremy Robertson;
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Department of Chemistry, University of Oxford, Chemistry Research Laboratory, Mansfield Road, Oxford, OX1 3TA, UK;

Department of Chemistry, University of Oxford, Chemistry Research Laboratory, Mansfield Road, Oxford, OX1 3TA, UK;

Department of Chemistry, University of Oxford, Chemistry Research Laboratory, Mansfield Road, Oxford, OX1 3TA, UK;

Department of Chemistry, University of Oxford, Chemistry Research Laboratory, Mansfield Road, Oxford, OX1 3TA, UK;

Department of Chemistry, University of Oxford, Chemistry Research Laboratory, Mansfield Road, Oxford, OX1 3TA, UK;

AstraZeneca Global R&D, Alderley Park, Macclesfield, Cheshire, SK10 4TG, UK;

Department of Chemistry, University of Oxford, Chemistry Research Laboratory, Mansfield Road, Oxford, OX1 3TA, UK;

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Rhodium(Ⅱ)-catalysed tandem aziridination and ring-opening: stereoselective synthesis of functionalised tetrahydrofurans

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